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| 1 | Weakening relationship between East Asian winter monsoon and ENSO after mid-1970s显示文摘The East Asian winter monsoon(EAWM) is characterized by the frequent cold surges and associated closely with the Siberia High,East Asian Trough,and high-level westerly jet stream.The ENSO cycle can modulate the EAWM since it has co-variability with the sea surface temperature over the Indo-Western-Pacific which can tune the land-sea thermal contrast for the EAWM.This paper,by analyzing the EAWM,ENSO,and associated atmosphere-ocean variability,documents the weakening of the EAWMENSO relationship after the 1970s.The significant out-of-phase inter-relationship is found to be diminished after the 1970s.Further study in this work suggests that the weakened co-variability of the tropical Indo-Western-Pacific climate associated with ENSO after the 1970s is partly responsible for the weakened inter-relationship.Meanwhile,the reduced EAWM interannual variability and northward retreat of the EAWM-associated climate variability are favorable to the weakened ENSO-EAWM connection. | WANG HuiJun HE ShengPing | 2012 | Chinese Science Bulletin2012，57，27： | 39 |
| 2 | The increase of snowfall in Northeast China after the mid-1980s显示文摘We studied long-term variation of winter snowfall in Northeast China (NEC) for 1951-2010. Results show that NEC snowfall increased about 20% during 1986-2010 relative to 1951-1985. Further investigation suggests that the snowfall increase is closely associated with weakening of the East Asian winter monsoon (EAWM). The physical processes were portrayed by this research. Weakening of EAWM led to weakened cold air flow from the north, thus resulted in the warming of the surface ocean along the Northeast Asia coast and more water vapor evaporated from the ocean surface to the atmosphere and further transported to NEC. Also, because of EAWM weakening, more water vapor from south, east and west of NEC was transported to NEC, increasing water vapor content and hence snowfall there. From an atmospheric circulation viewpoint, EAWM weakening strengthened convergence at low levels and divergence at high levels, thereby favoring increased vertical convection and snowfall. | WANG HuiJun ShengPing | 2013 | Chinese Science Bulletin2013，58，12： | 11 |
| 3 | Impacts of the Autumn Arctic Sea Ice on the Intraseasonal Reversal of the Winter Siberian High显示文摘During 1979–2015, the intensity of the Siberian high(SH) in November and December–January(DJ) is frequently shown to have an out-of-phase relationship, which is accompanied by opposite surface air temperature and circulation anomalies.Further analyses indicate that the autumn Arctic sea ice is important for the phase reversal of the SH. There is a significantly positive(negative) correlation between the November(DJ) SH and the September sea ice area(SIA) anomalies. It is suggested that the reduction of autumn SIA induces anomalous upward surface turbulent heat flux(SHF), which can persist into November, especially over the Barents Sea. Consequently, the enhanced eddy energy and wave activity flux are transported to mid and high latitudes. This will then benefit the development of the storm track in northeastern Europe. Conversely, when downward SHF anomalies prevail in DJ, the decreased heat flux and suppressed eddy energy hinder the growth of the storm track during DJ over the Barents Sea and Europe. Through the eddy–mean flow interaction, the strengthened(weakened)storm track activities induce decreased(increased) Ural blockings and accelerated(decelerated) westerlies, which makes the cold air from the Arctic inhibited(transported) over the Siberian area. Therefore, a weaker(stronger) SH in November(DJ) occurs downstream. Moreover, anomalously large snowfall may intensify the SH in DJ rather than in November. The ensemble-mean results from the CMIP5 historical simulations further confirm these connections. The different responses to Arctic sea ice anomalies in early and middle winter set this study apart from earlier ones. | Zhuozhuo L Shengping HE Fei LI Huijun WANG | 2019 | Advances in Atmospheric Sciences2019，36，2： | 10 |
| 4 | Teleconnection between Sea Ice in the Barents Sea in June and the Silk Road,Pacific–Japan and East Asian Rainfall Patterns in August显示文摘In contrast to previous studies that have tended to focus on the influence of the total Arctic sea-ice cover on the East Asian summer tripole rainfall pattern, the present study identifies the Barents Sea as the key region where the June sea-ice variability exerts the most significant impacts on the East Asian August tripole rainfall pattern, and explores the teleconnection mechanisms involved. The results reveal that a reduction in June sea ice excites anomalous upward air motion due to strong near-surface thermal forcing, which further triggers a meridional overturning wave-like pattern extending to midlatitudes.Anomalous downward motion therefore forms over the Caspian Sea, which in turn induces zonally oriented overturning circulation along the subtropical jet stream, exhibiting the east–west Rossby wave train known as the Silk Road pattern. It is suggested that the Bonin high, a subtropical anticyclone predominant near South Korea, shows a significant anomaly due to the eastward extension of the Silk Road pattern to East Asia. As a possible descending branch of the Hadley cell, the Bonin high anomaly ultimately triggers a meridional overturning, establishing the Pacific–Japan pattern. This in turn induces an anomalous anticyclone and cyclone pair over East Asia, and a tripole vertical convection anomaly meridionally oriented over East Asia. Consequently, a tripole rainfall anomaly pattern is observed over East Asia. Results from numerical experiments using version 5 of the Community Atmosphere Model support the interpretation of this chain of events. | Shengping HE Yongqi GAO Tore FUREVIK Huijun WANG Fei LI | 2018 | Advances in Atmospheric Sciences2018，35，1： | 9 |
| 5 | RuCl_3 anchored onto post-synthetic modification MIL-101(Cr)-NH_2 as heterogeneous catalyst for hydrogenation of CO_2 to formic acid显示文摘A series of efficient ruthenium chloride (RuCl_3)-anchored MOF catalysts,such as RuCl_3@MIL-101 (Cr)-Sal,and RuCl_3@MIL-101 (Cr)-DPPB, have been successfully synthesized by post-synthetic modification (PSM)of the terminal amino of MIL-101(Cr)-NH_2 with salicylaldehyde, 2-diphenylphosphinobenzaldehyde (DPPBde) and anchoring of Ru (Ⅲ) ions. The stronger coordination electron donor interaction between Ru (Ⅲ) ions and chelating groups in the RuCl_3@MIL-101 (Cr)-DPPB enhances its catalytic performance for CO_2 hydrogenation to formic acid. The turnover number (TON) of formic acid was up to 831 in reaction time of 2 h with dimethyl sulfoxide (DMSO) and water (H_2O) as mixed solvent, trimethylamine (Et_3N) as organic base, and PPh_3 as electronic additive. | Shengping Wang Shihui Hou Chao Wu Yujun Zhao Xinbin Ma | 2019 | Chinese Chemical Letters2019，30，2： | 5 |
| 6 | Interface tuning of Cu+/CuO by zirconia for dimethyl oxalate hydrogenation to ethylene glycol over Cu/SiO2 catalyst显示文摘An efficient ZrO2-doped Cu/SiO2 catalyst was fabricated through hydrolysis precipitation method(HP)and used to produce ethylene glycol(EG)through dimethyl oxalate(DMO)hydrogenation.The states for zirconia on copper catalyst and roles in DMO hydrogenation were investigated through various characterization tools,including N2 physical adsorption,XRD,H2-TPR,Methyl glycolate-TPD-MS,XPS,XAES as well.Compared with common ammonia evaporation and co-precipitation methods used in catalyst preparation,this HP method is found to effectively suppress the agglomeration and further size growth of copper nanoparticles by enhancing the interactions between copper and zirconia species.More importantly,uniform distribution of ZrO2 dopant is achieved due to the pseudo-homogeneous reactions in the mixing step of catalyst preparation.A proper amount of zirconium dopant helps achieve the desirable proportion of Cu+/(Cu++CuO)for surface copper species,especially promotes the production of Cu+species originated from Cu-ZrO2 species at the interface of copper and zirconia particles.In comparison with Cu+species formed from copper phyllosilicates reduction,the Cu+sites derived from Cu-ZrO2 species show higher adsorption ability of MG,an important intermediate species in ethylene glycol production.These adsorbed MG molecules further react with atomic hydrogen shifted from adjacent metallic copper surface,leading to a higher catalytic behavior.For the EG production via DMO hydrogenation,the turnover frequency(TOF)normalized by CuO species on CuZr/SiO2 catalyst is 1.8 times than that of traditional Cu/SiO2 counterpart.Due to the enhanced synergy effect between Cu+and Cuo active sites,a lower activation energy of ester hydrogenation on this ZrO2-doped Cu/SiO2 catalyst is believed to be responsible for the significant improvement. | Yujun Zhao Huanhuan Zhang Yuxi Xu Shengnian Wang Yan Xu Shengping Wang Xinbin Ma | 2020 | Journal of Energy Chemistry2020，29，10： | 5 |
| 7 | A Sequencing-Based Linkage Map of Cucumber显示文摘 | Zhou, Qian Miao, Han Li, Shuai Zhang, Shengping Wang, Ye Weng, Yiqun Zhang, Zhonghua Huang, Sanwen Gu, Xingfang | 2015 | Molecular Plant2015，8，6： | 4 |
| 8 | Effects of antiviral therapy on hepatitis B virus reactivation and liver function after resection or chemoembolization for hepatocellular carcinoma显示文摘 | Xiang‐Ming Lao Guangyu Luo Liang‐Tao Ye Cheng Luo Ming Shi Dian Wang Rongping Guo Minshan Chen Shengping Li Xiaojun Lin Yunfei Yuan | 2013 | Liver Int2013，，4： | 3 |
| 9 | Distribution of soil aggregates and organic carbon in deep soil under long-term conservation tillage with residual retention in dryland显示文摘To ascertain the effects of long-term conservation tillage and residue retention on soil organic carbon(SOC) content and aggregate distribution in a deep soil(>20-cm depth) in a dryland environment,this paper analyzed the SOC and aggregate distribution in soil, and the aggregate-associated organic carbon(OC) and SOC physical fractions. Conservation tillage(reduced tillage with residue incorporated(RT) and no-tillage with residue mulch(NT)) significantly increased SOC sequestration and soil aggregation in deep soil compared with conventional tillage with residue removal(CT). Compared with CT, RT significantly increased the proportion of small macroaggregates by 23%–81% in the 10–80 cm layer, and the OC content in small macroaggregates by 1%–58% in the 0–80 cm layer. RT significantly increased(by 24%–90%) the OC content in mineral-SOC within small macroaggregates in the 0–60 cm layer, while there was a 23%–80% increase in the 0–40 cm layer with NT. These results indicated that:(1) conservation tillage treatments are beneficial for soil aggregation and SOC sequestration in a deep soil in a dryland environment; and(2)the SOC in mineral-associated OC plays important roles in soil aggregation and SOC sequestration. In conclusion, RT with NT is recommended as an agricultural management tool in dryland soils because of its role in improving soil aggregation and SOC sequestration. | WANG Bisheng GAO Lili YU Weishui WEI Xueqin LI Jing LI Shengping SONG Xiaojun LIANG Guopeng CAI Dianxiong WU Xueping | 2019 | Journal of Arid Land2019，11，2： | 3 |
| 10 | New ZnCe catalyst encapsulated in SBA-15 in the production of 1,3-butadiene from ethanol显示文摘ZnO-CeO2/SBA-15 catalysts were prepared by two kinds of solid-state grinding method and used for the production of 1,3-butadiene(1,3-BD) from ethanol.A mixture of SBA-15(with or without organic template) and metal precursors were ground in solid-state.The obtained catalysts were characterized by TG,N2 adsorption-desorption,TEM,XRD,Py-FTIR and NH_3-TPD techniques.Superior dispersion of metal oxides and more exposed acid sites were achieved on the catalyst lOZn_1Ce_5-AS with the presence of organic template in SBA-15 during the solid-state grinding process.The catalytic performance was evaluated in a fixed-bed reactor and a 1,3-butadiene selectivity of as high as 45% is achieved.This is attributed to the coupling effect of Zn and Ce species in the mesopores of SBA-15,in which Zn promotes ethanol dehydrogenation and Ce enhances aldol-condensation,respectively.Additionally,solvent-free method inspires new catalyst synthesis strategy for the production of 1,3-butadiene from ethanol. | Yujun Zhao Sijia Li Zheng Wang Shengnian Wang Shengping Wang Xinbin Ma | 2020 | Chinese Chemical Letters2020，31，2： | 3 |
| 11 | Variation in Principal Modes of Midsummer Precipitation over Northeast China and Its Associated Atmospheric Circulation显示文摘This study documents the first two principal modes of interannual variability of midsummer precipitation over Northeast China(NEC) and their associated atmospheric circulation anomalies. It is shown that the first principal mode exhibits the largest amount of variability in precipitation over the south of NEC(referred to as the south mode), whereas the second principal mode behaves with the greatest precipitation anomaly over the north of NEC(referred to as the north mode). Further findings reveal that, through modulating moisture transportation and upper-and lower-troposphere divergence circulation as well as vertical movement over NEC, the anomalous northwestern Pacific anticyclone and the anticyclone centered over northern NEC exert the dominant influence on the south and north modes, respectively. Additionally, it is quantitatively estimated that water vapor across the southern boundary of NEC dominates the moisture budget for the south mode, while the north mode has a close connection with moisture through NEC's northern and western boundaries. Furthermore, the north(south) mode is strongly related to the intensity(meridional shift) of the East Asian westerly jet. | Tingting HAN Shengping HE Huijun WANG Xin HAO | 2019 | Advances in Atmospheric Sciences2019，36，1： | 3 |
| 12 | Pd-Fe/a-AI203/cordierite monolithic catalysts for the synthesis of dimethyl oxalate: effects of calcination and structure显示文摘 | Shengping WANG Xin ZHANG Yujun ZHAO Yadong GE Jing LV Baowei WANG Xinbin MA | 2012 | Frontiers of Chemical Science and Engineering2012，6，3： | 3 |
| 13 | Influence of crystalline phase of Li-AI-O oxides on the activity of Wacker-type catalysts in dimethyl carbonate synthesis显示文摘 | Yadong GE Yuanyuan DONG Shengping WANG Yujun ZHAO Jing LV Xinbin MA | 2012 | Frontiers of Chemical Science and Engineering2012，6，4： | 3 |
| 14 | Reconstruction clipping of ruptured anterior circulation aneurysms via supraorbital lateral keyhole approach显示文摘Background:Intracranial aneurysm(IA)is a serious disease.Analyze and review the cases of anterior circulation ruptured IA by supraorbital lateral keyhole approach,and summarize the experiences of this approach.Methods:Retrospective analysis of 16 cases of ruptured anterior circulation IA in our department from January 2019 to June 2020,CT angiography(CTA)was performed before operation.Analyzing the IA’s parameters by 3D-CT reconstruction.The IA was clipped by supraorbital lateral keyhole approach combined with the 3D-skull reconstruction.Extraventricular drainage was performed before craniotomy.Intraoperative neurophysiological monitoring was performed during the operation.After operation,fluorescein angiography and vascular ultrasound were performed to check the clipping effect.Intracranial pressure monitor was performed postoperatively.CTA was reexamined one week after operation.The modified Rankin Scale(MRS)was performed 6 months after operation.Results:There were 7 males(43.8%)and 9 females(56.2%),and the average age is 52.31±11.12 years old.Among them,11 patients(68.8%)were anterior communicating artery aneurysms and 5(31.2%)were middle cerebral artery aneurysms.All patients were out of hospital within 10 days without any death,without cerebral infarction,cerebrospinal fluid leakage and neurological impairments.About mRS score,after 6 months follow-up,8 cases(50%)had 0 point,4 cases(25%)had 1 point,and 4 cases(25%)had 2 points.Conclusions:For ruptured anterior circulation IA,the supraorbital lateral keyhole approach combined with ventricular drainage,intraoperative electrophysiological monitoring,and intraoperative vascular ultrasound is a safe and minimally invasive treatment.The application of reconstruction clipping can reconstruct the diameter of parent vessel and reduce the recurrence rate of IA. | Yuzhang Wu Yan Zhao Shengping Yu Fan Li Shifei Cai Chao Peng Zhen Wang Yifan Yang Bangyue Wang Xinyu Yang | 2022 | Chinese Neurosurgical Journal2022，8，2： | 2 |
| 15 | Effect of thermal pretreatment on the surface structure of PtSn/SiO2 catalyst and its performance in acetic acid hydrogenation显示文摘活跃地点和在醋酸(AcOH ) 的 PtSn/SiO 2 催化剂的催化表演上的热预告的处理的效果加氢在这篇文章被调查。催化剂被 N 2 描绘物理吸附, X 光检查衍射,传播电子显微镜学, pyridine Fourier 变换红外线的系列,和它的物理化学的性质上的 H 2-O2 滴定。结果证明那磅种首先在水晶的结构被形成,没有 PtSn x 合金被观察。与热预告的处理温度的增长,同时,磅分散由于磅粒子的聚集显示出一个减少的趋势。同时,路易斯酸地点的数量被拥有到 Sn 种类的作为结果的物理化学的性质变化的如此的热预告的处理显著地影响。有趣地,催化活动与路易斯酸地点的显示出类似的变化趋势,证实在 AcOH 加氢的路易斯酸地点的重要角色。而且,在暴露的磅和路易斯酸地点之间的平衡效果被获得,在 AcOH 加氢导致优异催化表演。 | Guozhen Xu Jian Zhang Shengping Wang Yujun Zhao Xinbin Ma | 2016 | Frontiers of Chemical Science and Engineering2016，10，3： | 2 |
| 16 | Connection between the Silk Road Pattern in July and the Following January Temperature over East Asia显示文摘This study investigates a cross-seasonal influence of the Silk Road Pattern(SRP)in July and discusses the related mechanism.Both the reanalysis and observational datasets indicate that the July SRP is closely related to the following January temperature over East Asia during 1958/59–2001/02.Linear regression results reveal that,following a higher-than-normal SRP index in July,the Siberian high,Aleutian low,Urals high,East Asian trough,and meridional shear of the East Asian jet intensify significantly in January.Such atmospheric circulation anomalies are favorable for northerly wind anomalies over East Asia,leading to more southward advection of cold air and causing a decrease in temperature.Further analysis indicates that the North Pacific sea surface temperature anomalies(SSTAs)might play a critical role in storing the anomalous signal of the July SRP.The significant SSTAs related to the July SRP weaken in October and November,re-emerge in December,and strengthen in the following January.Such an SSTA pattern in January can induce a surface anomalous cyclone over North Pacific and lead to dominant convergence anomalies over northwestern Pacific.Correspondingly,significant divergence anomalies appear,collocated in the upper-level troposphere in situ.Due to the advection of vorticity by divergent wind,which can be regarded as a wave source,a stationary Rossby wave originates from North Pacific and propagates eastward to East Asia,leading to temperature anomalies through its influence on the large-scale atmospheric circulation. | Shengping HE Yang LIU Huijun WANG | 2017 | Journal of Meteorological Research2017，31，2： | 2 |
| 17 | Oxycarbonylation of methanol over modified CuY: Enhanced activity by improving accessibility of active sites显示文摘CuY zeolite is a promising catalyst in the field of manufacturing dimethyl carbonate(DMC) through oxidative carbonylation of methanol. Cu^+ exchanged with Br?nsted acid sites are supposed to be active for this reaction. However, the location of Cu^+ in small cages can not interact with reactants because of steric hindrance, which lead to a waste of Cu species. In this work, NH_4F solution was used to modify the pore structure of zeolite Y by etching the framework T atoms. Physical and chemical adsorption of probe molecules with different size are used to determine the changes of porosity as well as the accessibility of Cu^+ sites. At an optimized etching time, the small cages were opened with maintained zeolitic framework. As a result, more Cu^+ species located in small cages become accessible to reactants, which contributes to the enhanced activity in this reaction. | Hexin Zhou Shengping Wang Baowei Wang Xinbin Ma Shouying Huang | 2019 | Chinese Chemical Letters2019，30，3： | 2 |
| 18 | Efficient MgO-doped CaO sorbent pellets for high temperature CO_(2) capture显示文摘Novel MgO-doped CaO sorbent pellets were prepared by gel-casting and wet impregnation.The effect of Na^(+) and MgO on the structure and CO_(2) adsorption performance of CaO sorbent pellets was elucidated.MgOdoped CaO sorbent pellets with the diameter range of 0.5-1.5 mm exhibited an excellent capacity for CO_(2) adsorption and adsorption rate due to the homogeneous dispersion of MgO in the sorbent pellets and its effects on the physical structure of sorbents.The results show that MgO can effectively inhibit the sintering of CaO and retain the adsorption capacity of sorbents during multiple adsorption-desorption cycles.The presence of mesopores and macropores resulted in appreciable change of volume from CaO(16.7 cm^(3)·mol^(-1))to CaCO3(36.9 cm^(3)·mol^(-1))over repeated operation cycles.Ca2Mg1 sorbent pellets exhibited favorable CO_(2) capture capacity(9.49 mmol·g^(-1)),average adsorption rate(0.32 mmol·g^(-1)·min^(-1)) and conversion rate of CaO(74.83%) after 30 cycles. | Zhihong Xu Tao Jiang Hao Zhang Yujun Zhao Xinbin Ma Shengping Wang | 2021 | Frontiers of Chemical Science and Engineering2021，15，3： | 2 |
| 19 | Tandem Biocatalysis by CotA-TJ102@UIO-66-NH2 and Novozym 435 for Highly Selective Transformation of HMF into FDCA显示文摘2,5-Furandicarboxylic acid (FDCA) is a potential biorenewable chemical for applications including plastics, polyamides, drugs, etc. The selective biosynthesis of FDCA from 5-hydroxymethylfurfural (HMF) by a speci c enzyme poses a great challenge. In this study, we reported an e cient strategy to produce FDCA from HMF by the tandem biocatalysis of laccase (CotA-TJ102@UIO-66-NH 2 ) and Novozym 435. For the rst step, a nanoparticle metal organic framework was synthesized as a carrier to immobilize CotA-TJ102@UIO-66-NH 2 , which was assigned for the production of 5-formyl-2-furancarboxylic acid (FFCA) and featured an enzyme loading of 255.54 mg/g, speci c activity of 135.90 U/mg, and solid loading ratio of 99.65%. Under optimal conditions, an ideal FFCA yield of 98.5% was achieved, and the CotA-TJ102@UIO-66-NH2 pre- sented a high recycling capacity after 10 cycles. For the second step, Novozym 435 was applied for the further conversion of FFCA into FDCA, presenting a high FDCA yield of 95.5% under the optimized conditions. Novozym 435 also exhibited a high recyclability after eight cycles. As a result, the tandem biocatalysis strategy provided a 94.2% FDCA yield from HMF, indicating its excellence as a method for FDCA production. | Xin Chang Chengyu Zhang Lan Gao Xiao Liu Shengping You Wei Qi Kang Wang Xin Guo Rongxin Su Han Lu Zhimin He | 2019 | Transactions of Tianjin University2019，25，5： | 2 |
| 20 | In-situ green synthesis of highly active GSH-capped Pt–Au–Ag-hybrid nanoclusters显示文摘Recently much attention has been paid to the application of metal hybrid nanoparticles in industrial catalytic fields because of their super-efficient catalytic activity and attractive properties. We explored a novel strategy to prepare GSH-capped Pt–Au–Ag-hybrid nanoclusters through the synergistic effect between ascorbic acid(VC) and glutathione(GSH) with chloroplatinic acid, chloroauric acid, and silver nitrate as precursors. The potential utilization of as-prepared GSH-capped Pt–Au–Aghybrid nanoclusters for catalytic applications has been evaluated through the reduction of 4-nitrophenol(4-NP) with NaBH4; we obtained the kinetic data by monitoring with UV-Vis spectroscopy. Our results illustrate that GSH-capped Pt–Au– Ag-hybrid nanoclusters could facilitate the process of reduction of 4-NP in a way that is unprecedented. This approach may offer a novel, non-cytotoxicity, efficient catalyst for industry. | CHEN DongHua GAO ShengPing UR REHMAN Fawad JIANG Hui WANG XueMei | 2014 | Science China Chemistry2014，57，11： | 2 |
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