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Distribution of polybrominated diphenyl ethers and decabromodiphenylethane in surface sediments from Fuhe River and Baiyangdian Lake,North China

查看全文 作  者:Guocheng [1,2]Hu;Zhencheng [1]Xu;Jiayin [2]Dai;Bixian [3]Mai;Hong [2]Cao;Jianshe [2]Wang;Zhimin [2]Shi;Muqi [2]Xu 高影响力作者 机构地区:[1]Metropolitan Environment Center, South China Institute of Environmental Sciences, Ministry of Environmental Protection, Guangzhou 510655, China;[2]Key Laboratory of Animal Ecology and Conservation Biology, Institute of Zoology, Chinese Academy of Sciences, Beijing 100101, China;[3]State Key Laboratory of Organic Chemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China高影响力机构 出  处:《Journal of Environmental Sciences》索引2010年第22卷第12期,共7页高影响力期刊 基  金:supported by the National Basic Research Program(973) of China(No. 2006CB403306);the National Natural Science Foundation of China(No.30870311) 摘  要:Nineteen surface sediment samples collected from Baiyangdian Lake and its inflowing river (Fuhe River) in North China were analyzed for polybrominated diphenyl ethers (PBDEs) and decabromodiphenylethane (DBDPE).The concentrations of PBDEs and DBDPE in sediments ranged from 5.5 to 300.7 ng/g dry weight (dw) and 1.1 to 68.2 ng/g dw,respectively.Their levels in sediments in Fuhe River were significantly higher than those in Baiyandian Lake.Compared to data from other regions,the PBDE levels in surface sediments from Baiyangdian Lake and Fuhe River were in the medium to lower range.Among the PBDE congeners,BDE209 was predominant,with contributions to the total PBDEs ranging from 79.4% to 97.3% in sediment samples.For the lowly brominated congeners (tri-to hepta-BDE),BDE47 and BDE99 were the most abundant,which contributed 52.1% and 44.1% to the sum of tri-to hepta-BDEs in the sediments from Baiyangdian Lake and Fuhe River,respectively.The compositional patterns of PBDEs in Baiyangdian Lake sediments indicated that technical deca-BDE mixture was the major pollutant sources with a minor contribution of penta-BDE mixture.The present study suggested that the importance of Fuhe River as a possibly potential sources of PBDEs contamination in Baiyangdian Lake. 关 键 词:十溴二苯乙烷 表层沉积物 多溴联苯醚 白洋淀 府河 中国 多溴二苯醚 PBDES
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