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Biological removal of antiandrogenic activity in gray wastewater and coking wastewater by membrane reactor process

查看全文 作  者:Dehua [1]Ma;Lujun [1,2]Chen;Cong [1]Liu;Chenjun [1]Bao;Rui [2]Liu 高影响力作者 机构地区:[1]School of Environment, Tsinghua University;[2]Zhejiang Provincial Key Laboratory of Water Science and Technology高影响力机构 出  处:《Journal of Environmental Sciences》索引2015年第27卷第7期,共8页高影响力期刊 基  金:funded by the National High-Tech Research and Development Program (863 Program) of China (No. 2013AA062705-1);the National Natural Science Funds of China (No. 51308319) 摘  要:A recombinant human androgen receptor yeast assay was applied to investigate the occurrence of antiandrogens as well as the mechanism for their removal during gray wastewater and coking wastewater treatment. The membrane reactor(MBR) system for gray wastewater treatment could remove 88.0% of antiandrogenic activity exerted by weakly polar extracts and 97.3% of that by moderately strong polar extracts, but only 32.5%of that contributed by strong polar extracts. Biodegradation by microorganisms in the MBR contributed to 95.9% of the total removal. After the treatment, the concentration of antiandrogenic activity in the effluent was still 1.05 μg flutamide equivalence(FEQ)/L, 36.2%of which was due to strong polar extracts. In the anaerobic reactor, anoxic reactor, and membrane reactor system for coking wastewater treatment, the antiandrogenic activity of raw coking wastewater was 78.6 mg FEQ/L, and the effluent of the treatment system had only 0.34 mg FEQ/L. The antiandrogenic activity mainly existed in the medium strong polar and strong polar extracts. Biodegradation by microorganisms contributed to at least 89.2%of the total antiandrogenic activity removal in the system. Biodegradation was the main removal mechanism of antiandrogenic activity in both the wastewater treatment systems. 关 键 词:焦化废水 抗雄激素 膜反应器 活性 水生物 膜生物反应器 微生物降解 反应器系统
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