维普中文期刊产品整合服务

Facile construction of highly efficient MOF-based Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)flower-like nanocomposites for visible-light-driven photocatalytic hydrogen production

查看全文 作　　者：Mengting [1]Cao;Fengli [1]Yang;Quan [1]Zhang;Juhua [1]Zhang;Lu [1]Zhang;Lingfeng [1]Li;Xiaohao [1]Wang;Wei-Lin [1]Dai 高影响力作者 机构地区：[1]Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials,Fudan University,Shanghai 200438,China高影响力机构 出　　处：《Journal of Materials Science & Technology》索引2021年第17期,共11页高影响力期刊 基　　金：the Natural Science Foundation of Shanghai(No.19ZR1403500);the National Natural Science Foundation of China(No.21373054);the Natural Science Foundation of Shanghai Science and Technology Committee(No.19DZ2270100)。 摘　　要：Construction of metal-organic-frame works-based composite photocatalysts has attracted much attention for the reasonable band gap and high surface areas to improve the photocatalytic activity.In this study,the ternary heterojunction Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)nanocomposites were facilely prepared for the first time by a two-step method.The visible-light-promoted hydrogen production rate of 0.3%Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)reaches up to 5.26 mmol g^(-1)h^(-1),which is evidently much higher than pure UiO-66-NH_(2),ZnIn_(2)S_(4)and binary UiO-66-NH_(2)/ZnIn_(2)S_(4)composites.Such a huge improvement in the photocatalytic performance is mainly attributed to the matched band gap of ZnIn_(2)S_(4)and UiO-66-NH_(2),and the introduction of Pd NPs into photocatalysts that broaden spectral response range and promote the photon induced charge carrier separation.This work may provide a feasible approach for the design and construction of metal-organic-frameworks-based photocatalytic materials. 关 键 词：Metal-organic frameworks(MOFs) UiO-66-NH_(2) ZnIn_(2)S_4 Pd nanoparticles Photocatalytic hydrogen production
相关文献

参考文献(63)

引证文献(5)

网站首页 | 关于我们 | 联系我们 | 产品服务 | 客服中心 | 广告服务 | 版权声明 | 网站联盟 | 友情链接 | 售卡网点

版权所有© 渝B2-20050021-1　渝公网安备 50019002500403号　违法和不良信息举报中心

互联网出版许可证 新出网证(渝)字10号 全国400电话 - 免长途话费