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A New Index Developed for Fast Diagnosis of Meteorological Roles in Ground-Level Ozone Variations

查看全文 作  者:Weihua [1]CHEN;Weiwen [1]WANG;Shiguo [2]JIA;Jingying [1]MAO;Fenghua [1]YAN;Lianming [1]ZHENG;Yongkang [1]WU;Xingteng [1]ZHANG;Yutong [1]DONG;Lingbin [1]KONG;Buqing [3]ZHONG;Ming [1]CHANG;Min [1]SHAO;Xuemei [1]WANG 高影响力作者 机构地区:[1]Guangdong-Hongkong-Macao Joint Laboratory of Collaborative Innovation for Environmental Quality,Institute for Environmental and Climate Research,Jinan University,Guangzhou 510632,China;[2]School of Atmospheric Sciences,Guangdong Province Key Laboratory for Climate Change and Natural Disaster Studies,Sun Yat-sen University,Guangzhou 510275,China;[3]Key Laboratory of Vegetation Restoration and Management of Degraded Ecosystems,South China Botanical Garden,Chinese Academy of Sciences,Guangzhou 510650,China高影响力机构 出  处:《Advances in Atmospheric Sciences》索引2022年第39卷第3期,共18页高影响力期刊 基  金:supported by the National Key Research and Development Plan(Grant No.2017YFC0210105);the second Tibetan Plateau Scientific Expedition and Research Program(Grant No.2019QZKK0604);the National Natural Science Foundation of China(Grant Nos.41905086,41905107,42077205,and 41425020);the Special Fund Project for Science and Technology Innovation Strategy of Guangdong Province(Grant No.2019B121205004);the China Postdoctoral Science Foundation(Grant No.2020M683174);the Air Quip(High-resolution Air Quality Information for Policy)Project funded by the Research Council of Norway;the Collaborative Innovation Center of Climate Change;Jiangsu Province;China;the high-performance computing platform of Jinan University。 摘  要:China experienced worsening ground-level ozone(O_(2)) pollution from 2013 to 2019. In this study, meteorological parameters, including surface temperature(T_(2)), solar radiation(SW), and wind speed(WS), were classified into two aspects,(1) Photochemical Reaction Condition(PRC = T_(2)× SW) and(2) Physical Dispersion Capacity(PDC = WS). In this way, a Meteorology Synthetic Index(MSI = PRC/PDC) was developed for the quantification of meteorology-induced ground-level O_(2)pollution. The positive linear relationship between the 90 th percentile of MDA8(maximum daily 8-h average) O_(2)concentration and MSI determined that the contribution of meteorological changes to ground-level O-3 varied on a latitudinal gradient, decreasing from ~40% in southern China to 10%–20% in northern China. Favorable photochemical reaction conditions were more important for ground-level O_(2)pollution. This study proposes a universally applicable index for fast diagnosis of meteorological roles in ground-level O_(2)variability, which enables the assessment of the observed effects of precursor emissions reductions that can be used for designing future control policies. 关 键 词:ground-level ozone meteorology synthetic index photochemical reaction condition physical dispersion capacity
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