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A study on wildfire impacts on greenhouse gas emissions and regional air quality in South of Orléans,France

查看全文 作  者:Chaoyang [1]Xue;Gisèle [1]Krysztofiak;Yangang [2,3]Ren;Min [2]Cai;Patrick [4]Mercier;Frédéric Le [4]Fur;Corinne [4]Robin;Benoit [2]Grosselin;Véronique [2]Daele;Max [2]RMcGillen;Yujing [3]Mu;Valéry [1]Catoire;Abdelwahid [2,5]Mellouki 高影响力作者 机构地区:[1]Laboratoire de Physique et Chimie de l’Environnement et de l’Espace(LPC2E),CNRS–UniversitéOrléans–CNES(UMR 7328),Orléans Cedex 245071,France;[2]Institut de Combustion,Aérothermique,RéactivitéEnvironnement(ICARE),CNRS,Orléans Cedex 245071,France;[3]Research Centre for Eco-Environmental Sciences,Chinese Academy of Sciences,Beijing 100085,China;[4]Lig’Air-Association de surveillance de la qualitéde l’air en région Centre-Val de Loire,Saint-Cyr-en-Val 45590,France;[5]Mohammed V University,Rabat,Morocco高影响力机构 出  处:《Journal of Environmental Sciences》索引2024年第1期,共13页高影响力期刊 基  金:supported by the VOLTAIRE project (ANR-10-LABX-100-01)funded by the ANR and the PIVOTS project provided by the Region Centre−Val de Loire (ARD 2020 program and CPER 2015−2020). 摘  要:Wildfire events are increasing globally which may be partly associated with climate change,resulting in significant adverse impacts on local,regional air quality and global climate.In September 2020,a small wildfire(burned area:36.3 ha)event occurred in Souesmes(Loiret-Cher,Sologne,France),and its plume spread out over 200 km on the following day as observed by the MODIS satellite.Based on measurements at a suburban site(~50 km northwest of the fire location)in Orléans and backward trajectory analysis,young wildfire plumes were characterized.Significant increases in gaseous pollutants(CO,CH_(4),N_(2)O,VOCs,etc.)and particles(including black carbon)were found within the wildfire plumes,leading to a reduced air quality.Emission factors,defined as EF(X)=ΔX/ΔCO(where,X represents the target species),of various trace gases and black carbon within the young wildfire plumes were determined accordingly and compared with previous studies.Changes in the ambient ions(such as ammonium,sulfate,nitrate,chloride,and nitrite in the particle-and gasphase)and aerosol properties(e.g.,aerosol water content,aerosol p H)were also quantified and discussed.Moreover,we estimated the total carbon and climate-related species(e.g.,CO_(2),CH_(4),N_(2)O,and BC)emissions and compared them with fire emission inventories.Current biomass burning emission inventories have uncertainties in estimating small fire burned areas and emissions.For instance,we found that the Global Fire Assimilation System(GFAS)may underestimate emissions(e.g.,CO)of this small wildfire while other inventories(GFED and FINN)showed significant overestimation.Considering that it is the first time to record wildfire plumes in this region,related atmospheric implications are presented and discussed. 关 键 词:WILDFIRE Air quality Emission factor Emission inventory VOLTAIRE supersite
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