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| 1 | Removal of antibiotics in a parallel-plate thin-film-photocatalytic reactor: Process modeling and evolution of transformation by-products and toxicity显示文摘Photocatalytic degradation of sulfamethoxazole(SMX) antibiotic has been studied under recycling batch and homogeneous flow conditions in a thin-film coated immobilized system namely parallel-plate(PPL) reactor. Experimentally designed, statistically evaluated with a factorial design(FD) approach with intent to provide a mathematical model takes into account the parameters influencing process performance. Initial antibiotic concentration, UV energy level, irradiated surface area, water matrix(ultrapure and secondary treated wastewater) and time, were defined as model parameters. A full of 2~5 experimental design was consisted of 32 random experiments. PPL reactor test experiments were carried out in order to set boundary levels for hydraulic, volumetric and defined defined process parameters. TTIP based thin-film with polyethylene glycol + TiO_2 additives were fabricated according to pre-described methodology. Antibiotic degradation was monitored by High Performance Liquid Chromatography analysis while the degradation products were specified by LC–TOF-MS analysis. Acute toxicity of untreated and treated SMX solutions was tested by standard Daphnia magna method. Based on the obtained mathematical model, the response of the immobilized PC system is described with a polynomial equation. The statistically significant positive effects are initial SMX concentration,process time and the combined effect of both, while combined effect of water matrix and irradiated surface area displays an adverse effect on the rate of antibiotic degradation by photocatalytic oxidation. Process efficiency and the validity of the acquired mathematical model was also verified for levofloxacin and cefaclor antibiotics. Immobilized PC degradation in PPL reactor configuration was found capable of providing reduced effluent toxicity by simultaneous degradation of SMX parent compound and TBPs. | Can Burak?zkal Zacharias Frontistis Maria Antonopoulou Ioannis Konstantinou Dionissios Mantzavinos Süreyya Meric | 2017 | Journal of Environmental Sciences2017，29，10： | 2 |
| 2 | Development and application of triglyceride 2-baaed polymers and composites显示文摘 | KHOT S N LASCALA J J CAN E | 2001 | J Appl Polyrn Sci2001，82，： | 1 |
| 3 | Rigid Thermosetting Liquid Molding Resins from Renewable Resources显示文摘 | CAN E WOOL S R P | 2002 | Journal of Applied Polymer Science2002，83，5： | 1 |
| 4 | Effects of dexmedetomidine or methylprednisolone on inflammatory responses in spinal cord injury显示文摘 | Can M Gul S Bektas S | 2009 | Acta Anaesthesiol Scand2009，53，8： | 1 |
| 5 | Complications associated with the ball,bar and Locator attachments for implant-supported overdentures显示文摘 | Cakarer S Can T Yaltirik M | | 0，，7： | 1 |
| 6 | Characterization of polyphenol oxidase from litchi pericarp using ( - ) - epicatechin as substrate 显示文摘 | Liu L Can S Xie B Sun Z Li X Miao W | 2007 | Journal of Agriculture and Food Chemistry2007，55，17： | 1 |
| 7 | The association between coronary atherosclerotic burden and asymmetric dimethylarginine,carotis intima media thickness and endothelial function显示文摘 | Can F Ziyrek M Erdem S | 2014 | Turk Kardiyol Dern Ars2014，12，： | 1 |
| 8 | Modulation of Na^+/H^+ exchange isoform mRNA expression in isolated rat hearts显示文摘 | Can XT Chakrabarti S Karmazyn M | 1999 | Am-J-Physiol1999，277，32： | 1 |
| 9 | Specific ablation of the apototic functions of cytochrome c reveals a differential requirement for cytochrome c and apaf-1 in apoptosis显示文摘 | Hao Z Gordorn S Can D | 2005 | Cell2005，121，4： | 1 |
| 10 | Concise review:human umbilical cord stroma with regard to the source of fetus-derived stem cel s显示文摘 | Can A Karahuseyinoglu S | | 0，，11： | 1 |
| 11 | ARGONAUTF4 control of locus-specific siRNA accumulation and DNA and histone methylation显示文摘 | Zilberman D Can X Jacobsen S E | 2003 | Science2003，299，5607： | 1 |
| 12 | Priming with EGFR tyrosine kinase inhibitor and EGF sensitizes ovarian cancer ceils to respond to chemotherapeutical drugs 显示文摘 | Can C Lu S Sowa A | 2008 | Cancer Letters2008，266，2： | 1 |
| 13 | Numerical Simulation of Residual Stress and Birefringence in The Precision Injec- tion Molding of Plastic Microlens Arrays显示文摘 | Can Weng W B Lee S To | 2009 | International Communications in Heat and Mass Transfer2009，36，： | 1 |
| 14 | Evaluation of chronic cough in children显示文摘 | Asilsoy S Bayram E Agin H Apa H Can D Gulle S | 2008 | Chest2008，134，6： | 1 |
| 15 | Response of terrestrial carbon uptake to climate interannual variability in China显示文摘 | Can M K Prince S D Li K | 2003 | Global Change Biology2003，9，4： | 1 |
| 16 | Effects of lipid sources in the diet of laying hens on the fatty acid profiles of egg yolks显示文摘 | OLIVEIRA D D BAIàO N C CAN?ADO S V | 2010 | Poultry Science2010，89，11： | 1 |
| 17 | Hemodynamic and hormonal stress responses to endotracheal tube and proSeal laryngeal Mask Air- way TM for laparoscopic gastric banding 显示文摘 | Can'on M Veronese S Gomiero W | 2012 | Anesthesiology2012，117，2： | 1 |
| 18 | Cystain C and neuropeptide Y levels in brain tissues after experimental subarachnoid hemorrhage 显示文摘 | ACIKGOZ S CAN M GUVEN B | 2014 | Acta Biochimica Polonica2014，61，4： | 1 |
| 19 | Concise review: human umbilical cord stroma with regard to the source of fetus- derived stem cells 显示文摘 | Can A Karahuseyinoglu S | 2007 | Stem Cells2007，25，： | 1 |
| 20 | Soft computing-based aggregation methods for human resource management显示文摘 | CANóS L LIERN V | 2008 | European Journal of Operational Research2008，189，3： | 1 |
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