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| 1 | Defect and Doping Co‑Engineered Non‑Metal Nanocarbon ORR Electrocatalyst显示文摘Exploring low-cost and earth-abundant oxygen reduction reaction(ORR)electrocatalyst is essential for fuel cells and metal–air batteries.Among them,non-metal nanocarbon with multiple advantages of low cost,abundance,high conductivity,good durability,and competitive activity has attracted intense interest in recent years.The enhanced ORR activities of the nanocarbons are normally thought to originate from heteroatom(e.g.,N,B,P,or S)doping or various induced defects.However,in practice,carbon-based materials usually contain both dopants and defects.In this regard,in terms of the co-engineering of heteroatom doping and defect inducing,we present an overview of recent advances in developing non-metal carbon-based electrocatalysts for the ORR.The characteristics,ORR performance,and the related mechanism of these functionalized nanocarbons by heteroatom doping,defect inducing,and in particular their synergistic promotion effect are emphatically analyzed and discussed.Finally,the current issues and perspectives in developing carbon-based electrocatalysts from both of heteroatom doping and defect engineering are proposed.This review will be beneficial for the rational design and manufacturing of highly efficient carbon-based materials for electrocatalysis. | Jian Zhang Jingjing Zhang Feng He Yijun Chen Jiawei Zhu Deli Wang Shichun Mu Hui Ying Yang | 2021 | Nano-Micro Letters2021，13，4： | 8 |
| 2 | ZIF-8/LiFePO4 derived Fe-N-P Co-doped carbon nanotube encapsulated Fe2P nanoparticles for efficient oxygen reduction and Zn-air batteries显示文摘Iron-based oxygen reduction reaction(ORR)catalysts have been the focus of research,and iron sources play an important role for the preparation of efficient ORR catalysts.Here,we successfully use LiFePO4 as ideal sources of Fe and P to construct the heteroatom doped Fe-based carbon materials.The obtained Fe-N-P co-doped coral-like carbon nanotube arrays encapsulated Fe2P catalyst(C-ZIF/LFP)shows very high half-wave potential of 0.88 V in alkaline electrolytes toward ORR,superior to Pt/C(0.85 V),and also presents a high half-wave potential of 0.74 V in acidic electrolytes,comparable to Pt/C(0.8 V).When further applied into a home-made Zn-air battery as cathode,a peak power density of 140 mW·cm^-2 is reached,exceeds commercial Pt/C(110 mW·cm^-2).Besides,it also presents exceptional durability and methanol resistance compared with Pt/C.Noticeably,the preparation method of such a high-performance catalyst is simple and easy to optimize,suitable for the large-scale production.What’s more,it opens up a more sustainable development scenario to reduce the hazardous wastes such as LiFePO4 by directly using them for preparing high-performance ORR catalysts. | Huihui Jin Huang Zhou Pengxia Ji Chengtian Zhang Jiahuan Luo Weihao Zeng Chenxi Hu Daping He Shichun Mu | 2020 | Nano Research2020，13，3： | 8 |
| 3 | Regional Characteristics and Causes of Haze Events in Northeast China显示文摘Northeast China experiences severe atmospheric pollution, with an increasing occurrence of heavy haze episodes. However, the underlying forces driving haze formation during different seasons are poorly understood. In this study, we explored the spatio-temporal characteristics and causes of haze events in Northeast China by combining a range of data sources(i.e., ground monitoring, satellite-based products, and meteorological products). It was found that the ‘Shenyang-Changchun-Harbin(SCH)'city belt was the most polluted area in the region on an annual scale. The spatial distribution of air quality index(AQI) values had a clear seasonality, with the worst pollution occurring in winter, an approximately oval-shaped polluted area around western Jilin Province in spring, and the best air quality occurring in summer and most of the autumn. The three periods that typically experienced intense haze events were Period I from mid-October to mid-November(i.e., late autumn and early winter), Period II from late-December to February(i.e., the coldest time in winter), and Period III from April to mid-May(i.e., spring). During Period I, strong PM_(2.5) emissions from seasonal crop residue burning and coal burning for winter heating were the dominant reasons for the occurrence of extreme haze events(AQI > 300). Period II had frequent heavy haze events(200 < AQI < 300) in the coldest months of January and February, which were due to high PM_(2.5) emissions from coal burning and vehicle fuel consumption, a lower atmospheric boundary layer, and stagnant atmospheric conditions. Haze events in Period III, with high PM_(10) concentrations, were primarily caused by the regional transportation of windblown dust from degraded grassland in central Inner Mongolia and bare soil in western Jilin Province. Local agricultural tilling could also release PM_(10) and enhance the levels of windblown dust from tilled soil. Better control of coal burning, fuel consumption, and crop residue burning in winter and autumn is urgently needed to address the haze problem in Northeast China. | CHEN Weiwei ZHANG Shichun TONG Quansong ZHANG Xuelei ZHAO Hongmei MA Siqi XIU Aijun HE Yuexin | 2018 | Chinese Geographical Science2018，28，5： | 7 |
| 4 | Highly sensitive wearable sensor based on a flexible multi-layer graphene film antenna显示文摘The use of advanced carbon nanomaterials for flexible antenna sensors has attracted great attention due to their outstanding electromechanical properties. However, carbon nanomaterial based composites have yet to overcome drawbacks, such as low conductivity and toughness. In this work, a flexible multi-layer graphene film(FGF) with a high conductivity of 10~6 S/m for antenna based wearable sensors is investigated. A 1.63 GHz FGF antenna sensor exhibits significantly high strain sensitivity of 9.8 for compressive bending and 9.36 for tensile bending, which is super than the copper antenna sensor(5.39 for compressive bending and 4.05 for tensile bending). Moreover, the FGF antenna sensor shows very good mechanical flexibility, reversible deformability and structure stability, and thus is well suited for applications like wearable devices and wireless strain sensing. | Danli Tang Qianlong Wang Zhe Wang Quantao Liu Bin Zhang Daping He Zhi Wu Shichun Mu | 2018 | Science Bulletin2018，63，9： | 7 |
| 5 | Design Engineering,Synthesis Protocols,and Energy Applications of MOF-Derived Electrocatalysts显示文摘The core reactions for fuel cells,rechargeable metal-air batteries,and hydrogen fuel production are the oxygen reduction reaction(ORR),oxygen evolution reaction(OER),and hydrogen evolution reaction(HER),which are heavily dependent on the efficiency of electrocatalysts.Enormous attempts have previously been devoted in non-noble electrocatalysts born out of metal-organic frameworks(MOFs)for ORR,OER,and HER applications,due to the following advantageous reasons:(i)The significant porosity eases the electrolyte diffusion;(ii)the supreme catalyst-electrolyte contact area enhances the diffusion efficiency;and(iii)the electronic conductivity can be extensively increased owing to the unique construction block subunits for MOFs-derived electrocatalysis.Herein,the recent progress of MOFs-derived electrocatalysts including synthesis protocols,design engineering,DFT calculations roles,and energy applications is discussed and reviewed.It can be concluded that the elevated ORR,OER,and HER performances are attributed to an advantageously well-designed high-porosity structure,significant surface area,and plentiful active centers.Furthermore,the perspectives of MOF-derived electrocatalysts for the ORR,OER,and HER are presented. | Amr Radwan Huihui Jin Daping He Shichun Mu | 2021 | Nano-Micro Letters2021，13，9： | 4 |
| 6 | Ultra-small platinum nanoparticles segregated by nickle sites for efficient ORR and HER processes显示文摘In the electrochemical process,Pt nanoparticles(NPs)in Pt-based catalysts usually agglomerate due to Oswald ripening or lack of restraint,ultimately resulting in reduction of the active sites and catalytic efficiency.How to uniformly disperse and firmly fix Pt NPs on carbon matrix with suitable particle size for catalysis is still a big challenge.Herein,to prevent the agglomeration and shedding of Pt NPs,Ni species is introduced and are evenly dispersed in the surface of carbon matrix in the form of Ni-N-C active sites(Ni ZIF-NC).The Ni sites can be used to anchor Pt NPs,and then effectively limit the further growth and agglomeration of Pt NPs during the reaction process.Compared with commercial Pt/C catalyst,Pt@Ni ZIF-NC,with ultralow Pt loading(7 wt%)and ideal particle size(2.3 nm),not only increases the active center,but also promotes the catalysis kinetics,greatly improving the ORR and HER catalytic activity.Under acidic conditions,its half-wave potential(0.902 V)is superior to commercial Pt/C(0.861 V),and the mass activity(0.38 A per mg Pt)at 0.9 V is 4.7 times that of Pt/C(0.08 A per mg Pt).Besides,it also shows outstanding HER performance.At 20 and 30 mV,its mass activity is even 2 and 6 times that of Pt/C,respectively.Whether it is under ORR or HER conditions,it still shows excellent durability.These undoubtedly indicate the realization of dual-functional catalysts with low-Pt and high-efficiency properties. | Lvhan Liang Huihui jin Huang Zhou Bingshuai Liu Chenxi Hu Ding Chen Jiawei Zhu Zhe Wang Hai-Wen Li Suli Liu Daping He Shichun Mu | 2022 | Journal of Energy Chemistry2022，31，2： | 2 |
| 7 | Blind Equalization of Nonlinear Communication Channels Using Recurrent Wavelet Neu- ral Networks 显示文摘 | He Shichun He Zhenya | 1997 | IEEE International Conference on Acousties Speech and Signal Processing Munich Ger- many1997，4，： | 1 |
| 8 | A new strategy to access Co/N co-doped carbon nanotubes as oxygen reduction reaction catalysts显示文摘Carbon nanotubes(CNTs),as one-dimensional nanomaterials,show great potential in energy conversion and storage due to their efficient electrical conductivity and mass transfer.However,the security risks,time-consuming and high cost of the preparation process hinder its further application.Here,we develop that a negative pressure rather than a following gas environment can promote the generation of cobalt and nitrogen co-doped CNTs(Co/N-CNTs) by using cobalt zeolitic imidazolate framework(ZIF-67) as a precursor,in which the negative pressure plays a key role in adjusting the size of cobalt nanoparticles and stimulating the rearragement of carbon atoms for forming CNTs.Importantly,the obtained Co/N-CNTs,with high content of pyridinic nitrogen and abundant graphitized structure,exhibit superior catalytic activity for oxygen reduction reaction(ORR) with half-wave potential(E_(1/2)) of 0.85 V and durability in terms of the minimum current loss(2%) after the 30,000 s test.Our development provides a new pathway for large-scale and cost-effective preparation of metal-doped CNTs for various applications. | Bingshuai Liu Huang Zhou Huihui Jin Jiawei Zhu Zhe Wang Chenxi Hu Lvhan Liang Shichun Mu Daping He | 2021 | Chinese Chemical Letters2021，32，1： | 1 |
| 9 | Factors that influence carbon emissions due to energy consumption in China: Decomposition analysis using LMDI 显示文摘 | Shichun Xu Zhengxia He Ruyin Long | 2014 | Applied Energy2014，127，： | 1 |
| 10 | Porous graphene supported Pt catalysts for proton exchange membrane fuel cells显示文摘 | Kun Cheng Daping He Tao Peng Haifeng Lv Mu Pan Shichun Mu | 2014 | Electrochimica Acta2014，，： | 1 |
| 11 | CXCR-7 receptor promotes SDF-1α-induced migration of bone marrow mesenchymal stem cells in the transient cerebral ischemia/reperfusion rat hippocampus显示文摘 | Yulan Wang Wei Fu Shichun Zhang Xiaomei He Zhi’an Liu Diansuai Gao Tiejun Xu | 2014 | Brain Research2014，，： | 1 |
| 12 | Research on pumped two-phase single-sided cold plate of IGBT for rail transit applications显示文摘The use of pumped two-phase cooling to improve the thermal management of insulated gate bipolar transistor(IGBT)in rail transportation is a novel cooling technology.An experimental investigation on pumped two-phase cold plate of IGBT used in HXD1C locomotives was conducted at a mass flow rate of 0.1 kg/s–0.29 kg/s and a heat flux of 6.2 W/cm^(2),with R245fa as the working fluid.The experimental results showed that the base temperature nonuniformity can be controlled within 2.2℃ at flow rates of 0.14 kg/s and 0.19 kg/s,which is of great benefit to the reliability of IGBT.Based on well known correlations for saturated flow boiling in tubes,an analytical model was developed and compared with the experimental data.The model could predict the base temperature data within an error band of±3℃,as well as capture the trend of base temperature as a function of vapour quality and mass flow rate.The performance of the pumped two-phase cold plate of IGBT could be further improved with the aid of the developed model. | Hui Wu Gang Zhang Zhaozan Feng Kai He Lei Yao Wei Li Shichune Yao | 2021 | Transportation Safety and Environment2021，3，3： | 0 |
| 13 | 射频超导腔体在线清洗显示文摘In 2018,detailed studies on RF induced plasma for the in-situ cleaning of the HWR cavity were conducted to improve the performance of the cavity.For the purpose of cleaning the HWR cavities in cryomodule,an apparatus for the discharge experiments was designed at room temperature,which duplicates the assembly of cavities inside cryomodule,where the FPC was used for power coupling. | Wu Andong Huang Shichun Yang Lei Hua Chuanfei Li Chunlong Tan Teng Xiong Pingran Guo Hao Yue Weiming Pan Feng Chen Long Zhang Shenghu He Yuan Zhao Hongwei | 2018 | IMP & HIRFL Annual Report2018，，1： | 0 |
| 14 | Optimization of the Coating Process for Nbg_(3)Sn Cavity显示文摘After many years of worldwide exploration and improvement of the post treatment process,niobium(Nb)cavities are now approaching their fundamental limits both in terms of maximum acceleration field and in terms of surface resistance at typical operating temperatures. | Yang Ziqin He Yuan You Zhiming Guo Hao Xiong Pingran Song Yukun Zhang Shengxue Lu Ming Lin Zeqiang Huang Shichun Wu Andong Chu Qingwei Tan Teng Pan Feng Zhang Shenghu | 2019 | IMP & HIRFL Annual Report2019，，1： | 0 |
| 15 | 6-5 Operation of HWRs for C-ADS Injector显示文摘There are two types of HWR cavities have been developed in IMP for C-ADS Injector.HWR010s have been used to accelerate proton from 2.1 MeV to 10 MeV.There are 12 HWR010s assembled in two CMs.The taper type HWR015s have been used to accelerate proton from 10MeV to 18.5 MeV.There are 5 HWRs assembled in the third CM.Proton beam has been accelerated to 26 MeV by HWR010,HWR015 and Spoke021 in June 2017.The beam has been accelerated to 18.5 MeV by HWR010 and HWR015.The CMs in the tunnel are shown in Fig.1. | Yue Weiming Zhang Shenghu Li Yongming Chang Wei Jiang Tiancai Zhang Shengxue Gao Zheng Wang Ruoxue Huang Shichun Pan Feng Chen Long Li Chunlong Song Yukun Guo Hao Xiong Pingran Cong Zhang Tan Teng Wan Yuqin Niu Xiaofei Bai Feng Hu Chuanfei Zhang Peng Liu Lubei Huang Yulu Zhao Yugang Guo Xiaohong You Zhiming Zhang Junhui Huang Guirong He Yuan | 2016 | IMP & HIRFL Annual Report2016，，1： | 0 |
| 16 | 6-6 Nb/Cu SRF Cavity R&D Activity at IMP显示文摘SRF cavities are operated at Meissner state,which al-lows the electro-magnetic wave only interacts with the very surface of the cavity.The penetration depth of Nb at 4.2 is^100 nm,which means more than 99%of the expensive SRF grade Nb used on the SRF cavity is not involved in the interaction with the E-M wave.Fig.1 shows the schematics diagram of the interac-tion between magnetic field and a Nb coated Cu cavity.With a Nb film thicker than 3λ,the copper hide behind wouldn't be able to see the E-M wave nor generate RF dissipation. | Tan Teng Pan Feng Huang Shichun Zhang Cong Chu Qingwei He Yuan Zhao Hongwei | 2016 | IMP & HIRFL Annual Report2016，，1： | 0 |
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