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| 1 | Ultra-stable CsPbBr3 Perovskite Nanosheets for X-Ray Imaging Screen显示文摘Wet chemistry methods,including hot-injection and precipitation methods,have emerged as major synthetic routes for high-quality perovskite nanocrystals in backlit display and scintillation applications.However,low chemical yield hinders their upscale production for practical use.Meanwhile,the labile nature of halide-based perovskite poses a major challenge for long-term storage of perovskite nanocrystals.Herein,we report a green synthesis at room temperature for gram-scale production of CsPbBr3 nanosheets with minimum use of solvent,saving over 95% of the solvent for the unity mass nanocrystal production.The perovskite colloid exhibits record stability upon long-term storage for up to 8 months,preserving a photoluminescence quantum yield of 63% in solid state.Importantly,the colloidal nanosheets show self-assembly behavior upon slow solidification,generating a crack-free thin film in a large area.The uniform film was then demonstrated as an efficient scintillation screen for X-ray imaging.Our findings bring a scalable tool for synthesis of high-quality perovskite nanocrystals,which may inspire the industrial optoelectronic application of large-area perovskite film. | Liangling Wang Kaifang Fu Ruijia Sun Huqiang Lian Xun Hu Yuhai Zhang | 2019 | Nano-Micro Letters2019，11，3： | 4 |
| 2 | Better prognostic determination of cT3 rectal cancer through measurement of distance to mesorectal fascia:A multicenter study显示文摘Objective:To forward the magnetic resonance imaging(MRI)based distance between the deepest tumor invasion and mesorectal fascia(DMRF),and to explore its prognosis differentiation value in cT3 stage rectal cancer with comparison of cT3 substage.Methods:This was a retrospective,multicenter cohort study including cT3 rectal cancer patients undergoing neoadjuvant chemoradiotherapy followed by radical surgery from January 2013 to September 2014.DMRF and cT3 substage were evaluated from baseline MRI.The cutoff of DMRF was determined by disease progression.Multivariate cox regression was used to test the prognostic values of baseline variables.Results:A total of 804 patients were included,of which 226(28.1%)developed progression.A DMRF cutoff of7 mm was chosen.DMRF category,the clock position of the deepest position of tumor invasion(CDTI)and extramural venous invasion(EMVI)were independent predictors for disease progression,and hazard ratios(HRs)were 0.26[95%confidence interval(95%CI),0.13-0.56],1.88(95%CI,1.33-2.65)and 1.57(95%CI,1.13-2.18),respectively.cT3 substage was not a predictor for disease progression.Conclusions:The measurement of DMRF value on baseline MRI can better distinguish cT3 rectal cancer prognosis rather than cT3 substage,and was recommended in clinical evaluation. | Xiaoyan Zhang Qiaoyuan Lu Xiangjie Guo Wuteng Cao Hongmei Zhang Tao Yu Xiaoting Li Zhen Guan Xueping Li Ruijia Sun Yingshi Sun | 2021 | Chinese Journal of Cancer Research2021，33，5： | 1 |
| 3 | X-ray imager of 26-μm resolution achieved by perovskite assembly显示文摘Spatial resolution is an important criterion to evaluate the performance of a scintillation screen for X-ray imaging.Perovskite-based X-ray screen,usually made of powders or polycrystalline films,suffers from low spatial resolution(~200μm)due to the large thickness of scintillation layer despite of their compelling sensitivity to X-ray dose.In this work,a concentrated colloid of CsPbBr_(3)nanosheets was synthesized via a co-precipitation method at ambient condition.By drop casting,smooth scintillation screens of varied thickness were formed through self-assembly,which exhibited both high internal and external photoluminescence quantum yield(PL QY)(84.5%and 75.1%,respectively).The screen-based X-ray detector showed a high sensitivity down to 27 nGy/s,two orders of magnitude lower than the regular dose for medical diagnostics.Importantly,the screen of optimal thickness of 15μm showcased an unprecedented spatial resolution(26μm)when used for X-ray radiography,representing one order of magnitude improvement in perovskite community. | Zhaofen Wang Ruijia Sun Nianqiao Liu Huailin Fan Xun Hu Depeng Shen Yuhai Zhang Hong Liu | 2022 | Nano Research2022，15，3： | 1 |
| 4 | High-Performance Blue Quasi-2D Perovskite Light-Emitting Diodes via Balanced Carrier Confinement and Transfer显示文摘Extensive investigation of the passivating agents has been performed to suppress the perovskite defects.However,very few attentions have been paid to rationally design the passivating agents for the balance of the carrier confinement and transfer in quasi-2D perovskites,which is essential to achieve high-performance perovskite LEDs(PeLEDs).In this work,tributylphosphine oxide(TBPO)with moderate carbon chain length is demonstrated as a decent passivator for the quasi-2D perovskites by strengthening the carrier confinement for massive radiative recombination within the perovskites,and more importantly providing efficient carrier transfer in the quasi-2D perovskites.Benefiting from these interesting optoelectronic properties of TBPO-incorporated perovskites,we achieve high-efficient blue PeLEDs with an external quantum efficiency up to 11.5%and operational stability as long as 41.1 min without any shift of the electroluminescence spectra.Consequently,this work contributes an effective approach to promote the carrier confinement and transfer for high-performance and stable blue PeLEDs. | Zhenwei Ren Jiayun Sun Jiahao Yu Xiangtian Xiao Zhaojin Wang Ruijia Zhang Kai Wang Rui Chen Yu Chen Wallace C.H.Choy | 2022 | Nano-Micro Letters2022，14，4： | 1 |
| 5 | Deep learning model improves radiologists'performance in detection and classification of breast lesions显示文摘Objective:Computer-aided diagnosis using deep learning algorithms has been initially applied in the field of mammography,but there is no large-scale clinical application.Methods:This study proposed to develop and verify an artificial intelligence model based on mammography.Firstly,mammograms retrospectively collected from six centers were randomized to a training dataset and a validation dataset for establishing the model.Secondly,the model was tested by comparing 12 radiologists’performance with and without it.Finally,prospectively enrolled women with mammograms from six centers were diagnosed by radiologists with the model.The detection and diagnostic capabilities were evaluated using the freeresponse receiver operating characteristic(FROC)curve and ROC curve.Results:The sensitivity of model for detecting lesions after matching was 0.908 for false positive rate of 0.25 in unilateral images.The area under ROC curve(AUC)to distinguish the benign lesions from malignant lesions was0.855[95%confidence interval(95%CI):0.830,0.880].The performance of 12 radiologists with the model was higher than that of radiologists alone(AUC:0.852 vs.0.805,P=0.005).The mean reading time of with the model was shorter than that of reading alone(80.18 s vs.62.28 s,P=0.032).In prospective application,the sensitivity of detection reached 0.887 at false positive rate of 0.25;the AUC of radiologists with the model was 0.983(95%CI:0.978,0.988),with sensitivity,specificity,positive predictive value(PPV),and negative predictive value(NPV)of94.36%,98.07%,87.76%,and 99.09%,respectively.Conclusions:The artificial intelligence model exhibits high accuracy for detecting and diagnosing breast lesions,improves diagnostic accuracy and saves time. | Yingshi Sun Yuhong Qu Dong Wang Yi Li Lin Ye Jingbo Du Bing Xu Baoqing Li Xiaoting Li Kexin Zhang Yanjie Shi Ruijia Sun Yichuan Wang Rong Long Dengbo Chen Haijiao Li Liwei Wang Min Cao | 2021 | Chinese Journal of Cancer Research2021，33，6： | 1 |
| 6 | Coal rock image recognition method based on improved CLBP and receptive field theory显示文摘Rapid coal-rock identification is one of the key technologies for intelligent and unmanned coal mining.Currently,the existing image recognition algorithms cannot satisfy practical needs in terms of recognition speed and accuracy.In view of the evident differences between coal and rock in visual attributes such as color,gloss and texture,the complete local binary pattern(CLBP)image feature descriptor is introduced for coal and rock image recognition.Given that the original algorithm oversimplifies local texture features by ignoring imaging information from higher-order pixels and the concave and convex areas between adjacent sampling points,this paper proposes a higher-order differential median CLBP image feature descriptor to replace the original CLBP center pixel gray with a local gray median,and replace the binary differential with a second-order differential.Meanwhile,for the high dimensionality of CLBP descriptor histogram and feature redundancy,deep learning perceptual field theory is introduced to realize data nonlinear dimensionality reduction and deep feature extraction.With relevant experiments conducted,the following conclusion can be drawn:(1)Compared with that of the original CLBP,the recognition accuracy of the improved CLBP algorithm is greatly improved and finally stabilized above 94.3%under strong noise interference;(2)Compared with that of the original CLBP model,the single image recognition time of the coal rock image recognition model fusing the improved CLBP and the receptive field theory is 0.0035 s,a reduction of 71.0%;compared with the improved CLBP model(without the fusion of receptive field theory),it can shorten the recognition time by 97.0%,but the accuracy rate still maintains more than 98.5%.The method offers a valuable technical reference for the fields of mineral development and deep mining. | Chuanmeng Sun Ruijia Xu Chong Wang Tiehua Ma Jiaxin Chen | 2022 | Deep Underground Science and Engineering2022，1，2： | 0 |
| 7 | Preparation of V2O5 Porous Hollow Spheres and Study on Excellent Cycling Stability of Lithium Battery显示文摘Through one-step simple polyol-assisted (ethylene glycol) process, V2O5 hollow mi-cro-spheres about 3 micrometres in size were successfully synthesized. The structure is neat, the outer wall were porous. Testing its electrochemical properties with V2O5 hollow materials as cathode materia of lithium ion battery, the results showed that under the ratio of 1 C, the initial charge and discharge specific capacity were 236.8 mAh g^-1, 213 mAh g^-1, even if after 100 cycles, the charge and discharge specific capacity were still 220 mAh g^-1 and 219.7 mAh g^-1 respectively. Relative to the charge and discharge capacity of the second cycle, the keep rate were 93.2%, 92.9% respectively, has good cycle stability. | Shimeng Zhang Hongye Guan Dapeng Li Gengxin Zhang Ruijia Yang Liang Zhao Haibin Sun Zhicheng Lu Jiacai Wen Yujuan Dong | 2018 | Modern Electronic Technology2018，2，3： | 0 |
| 8 | A sustainable process to 100%bio-based nylons integrated chemical and biological conversion of lignocellulose显示文摘Considerable progress has been made in recent years to the development of sustainable polymers from bio-based feedstocks.In this study,100%bio-based nylons were prepared via an integrated chemical and biological process from lignocellulose.These novel nylons were obtained by the melt polymerization of 3-propyladipic acid derived from lignin and 1,5-pentenediamine/1,4-butanediamine derived from carbohydrate sugar.Central to the concept is a three-step noble metal free catalytic chemical funnelling sequence(Raney Ni mediated reductive catalytic fractionation-reductive funnelling-oxidative funnelling),which allowed for obtaining a single component 3-propyladipic acid from lignin with high efficiency.The structural and thermodynamic properties of the obtained nylons have been systematically investigated,and thus obtained transparent bio-based nylons exhibited higher Mw(>32,000)and excellent thermal stability(Td5%>265℃).Considering their moderate Tg and good melt strength,these transparent bio-based nylons could serve as promising functional additives or temperature-responsive materials. | Ruijia Hu Ming Li Tao Shen Xin Wang Zhuohua Sun Xinning Bao Kequan Chen Kai Guo Lei Ji Hanjie Ying Pingkai Ouyang Chenjie Zhu | 2024 | Green Energy & Environment2024，9，2： | 0 |
| 9 | Investigation and Protection of Fishery Resources in the Middle of Bohai Sea显示文摘In May and October 2017,12 stations were set up in the Central Bohai Sea for fishery resources investigation.The results show that there are many dominant species in this area,and the inshore fishery resources are higher than those in the open sea because of the abundant nutrients from land,the high density of zooplankton and the food of swimming animals.In order to effectively protect the fishery resources in the Central Bohai Sea,this paper puts forward some suggestions,such as strengthening the protection propaganda,scientific and reasonable fishing,and strengthening the management of marine environment. | Ruijia Zhou Xiao Liu Yiting Liu Mengmeng Bao Beibei Sun Xiaoyuan Du | 2021 | Journal of Fisheries Science2021，3，2： | 0 |
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