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| 1 | Asymmetric Transfer and Pressure Hydrogenation with Earth-Abundant Transition Metal Catalysts显示文摘 | Zhenfeng Zhang Nicholas Andrew Butt Muxing Zhou Delong Liu Wanbin Zhang | 2018 | Chinese Journal of Chemistry2018，36，5： | 8 |
| 2 | Ir-Catalyzed Asymmetric Hydrogenation of α-Alkylidene β-Lactams and Cyclobutanones显示文摘 | Jingzhao Xia Yu Nie Guoqiang Yang Yangang Liu Ilya D. Gridnev Wanbin Zhang | 2018 | Chinese Journal of Chemistry2018，36，7： | 3 |
| 3 | Highly stable and antifouling graphene oxide membranes prepared by bio-inspired modification for water purification显示文摘Graphene oxide(GO)membranes show great potential in molecular separation for water treatment.However,the inferior stability of GO membranes is a major bottleneck for practical applications.In this study,bio-inspired polydopamine(PDA)deposition is reported for enhancing the stability of GO membranes.Through simple and mild immersion,PDA is self-polymerized on GO membranes.The blocking of PDA chains to membrane defects improves the rejections for various molecules.Because the inherently strong adhesion and crosslinking of PDA greatly strengthen the interactions of substrates to GO layers and the binding force of GO nanosheets,the prepared PDA-GO membranes exhibit impressive long-te rm stability in cross-flow filtration,and maintain good nanofiltration perfo rmance at various feed pressures,tangential velocities,and eve n after external scratching.Moreover,because the deposited PDA layers obstruct the direct contact between GO and contaminants,the antifouling property of the PDA-GO membranes increases substantially,with recovery ratio about 98%. | Weiming Zhong Yuyu Zhang Ling Zhao Wanbin Li | 2020 | Chinese Chemical Letters2020，31，10： | 3 |
| 4 | Synergistic catalysis for stereocontrol of prochiral nucleophiles in palladium-catalyzed asymmetric allylic substitution显示文摘In contrast to the stereocontrol of the stereocenter at the allyl unit,the asymmetric induction of prochiral nucleophiles remains a challenge in Pd-catalyzed asymmetric allylic substitutions due to the remote distance between the chiral catalyst and the stereocenter established at prochiral nucleophile.Much effort has been devoted to solving this challenge through the elaborate design of chiral ligands.Recently,synergistic catalysis has gained increasing attention owing to its potential advantages over the traditional single palladium catalysis,such as improvement of reactivity and selectivity.This strategy,including bimetallic catalysis and Pd/organocatalysis,not only broadens the scope of prochiral nucleophiles,but also provides a simple and unified method for the stereocontrol of prochiral nucleophiles.This review summarizes the brief history and advances in this field. | Xi Wang Youbin Peng Ling Zhao Xiaohong Huo Wanbin Zhang | 2023 | Science China Chemistry2023，66，8： | 1 |
| 5 | Ni-Catalyzed Enantioconvergent Coupling of Epoxides with Alkenylboronic Acids:Construction of Oxindoles Bearing Quaternary Carbons显示文摘We have developed a nickel-nickel/bisphosphinecatalyzed stereoconvergent cross-coupling reaction of epoxides with alkenylboronic acids.Racemic spiroepoxyoxindoles were converted to chiral homoallylic alcohols bearing quaternary carbon stereogenic centers via a stereoablative enantioconvergent transformation.The subsequently fabricated oxindoles-carrying quaternary carbon products were obtained in good yields and enantioselectivity.A wide range of substrates and alkenylboronic acids was tolerated under the catalytic system.This reaction provided a rare example of a nickelcatalyzed enantioselective cross-coupling reaction of tertiary alkyl electrophiles and an enantioconvergent transformation of racemic epoxides,beneficial as a low-cost,sustainable,and efficient catalyst in the preparation of chiral oxindole-containing natural and pharmaceutical compounds. | Liang Wu Guoqiang Yang Wanbin Zhang | 2020 | CCS Chemistry2020，2，2： | 1 |
| 6 | Asymmetric Synthesis of Anti-tuberculosis-specific Drug TBAJ-876 through Synergistic Li/Li Catalysis显示文摘TBAJ-876, developed by TB Alliance, a novel anti-tuberculosis-specific drug, has entered Phase II clinical trials. Herein, the first asymmetric synthesis of TBAJ-876 has been realized using synergistic Li/Li catalysis with excellent yield of 95% and 88 : 12 er (99.6 : 0.4 er, 10 : 1 dr after simple recrystallization). Furthermore, DFT calculations and 7Li-NMR analysis illustrated the mechanism of the synergistic reaction: a chiral Li-complex activates the nucleophile to control the stereoselectivity, while the other achiral Li-complex activates the electrophile to catalyze the carbonyl addition reaction. Additionally, this protocol has been successfully carried out at 5 gram-scale, showing its industrial potential. | Jing Li Feng Gao Tanveer Ahmad Yicong Luo Zhenfeng Zhang Qianjia Yuan Wanbin Zhang | 2023 | Chinese Journal of Chemistry2023，41，11： | 1 |
| 7 | Novel hydrolyzable and biodegradable cationic gemini surfactants: bis ( ester - ammonium) dichloride having a butenylene or a butynylene spacer显示文摘 | TAIGA TATSUMI ZHANG WANBIN TOSHIYUKI KIDA | 2001 | Journal of Surfactants and Detergents2001，4，3： | 1 |
| 8 | Novel hydrolyzable and biodegradable cationic gemini surfactants : 1,3 - bis - 2 - hydroxypropane dichloride 显示文摘 | TAIGA TATSUMI ZHANG WANBIN TOSHIYUKI KIDA | 2000 | Journal of Surfactants and Detergents2000，3，2： | 1 |
| 9 | Novel hydrolyzable and biodegradable cationic gemini surfactants : Bis ( ester - ammonium) dichloride having a butenylene or a butynylene spacer 显示文摘 | TAIGA TATSUMI WANBIN ZHANG TOSHIYUKI K1DA | 2001 | Journal of Surfactants and Detergents2001，4，3： | 1 |
| 10 | Novel hydrolysable and biodegradable cationic gemini surfactants:1,3–bis(2 hydroxypropane dichloride显示文摘 | Taiga Tatsumi Wanbin Zhang Toshiyuki Kida Yohji Nakatsuji Daisuke Ono Tokuji Taketa Isao Ikeda | 1999 | J Surfact And Deterg1999，，： | 1 |
| 11 | Asymmetric synthesis of bedaquiline based on bimetallic activation and non-covalent interaction promotion strategies显示文摘Bedaquiline(BDQ),approved by Food and Drug Administration(FDA)in 2012 as the first anti-tuberculosis-specific drug in the last 40 years,is viewed as one of the world’s most promising treatments for tuberculosis(TB).Due to the stereoselective construction of the Csp^(3)–Csp^(3)bond with vicinal stereocenters of BDQ and its analogues being an unsolved challenge,there have not been any reports concerning its asymmetric synthesis for the current industrial production process until now.Herein,we have successfully developed a cooperative bimetallic system for the asymmetric synthesis of BDQ under the guidance of density functional theory(DFT)computations.Based on the optimized conditions,BDQ could be synthesized with excellent enantioselectivity(>99%ee)and diastereoselectivity(16:1 dr).A 5-g scale reaction was also conducted with comparably excellent results,showing its potential for industrial application. | Feng Gao Jing Li Tanveer Ahmad Yicong Luo Zhenfeng Zhang Qianjia Yuan Xiaohong Huo Tao Song Wanbin Zhang | 2022 | Science China Chemistry2022，65，10： | 1 |
| 12 | One Stone Two Birds-Enantioselective Bimetallic Catalysis forα-Amino Acid Derivatives with an Allene Unit显示文摘Main observation and conclusion A highly enantioselective 2,3-allenylation of acyclic and cyclicα-imino carboxylates via a synergistic bimetallic Pd/Cu catalysis with the same commercially available(R,Rp)-iPr-FOXAP(also as Phosferrox,(R,R)-[2-(4’-i-propyloxazolin-2’-yl)ferrocenyl]diphenyl phosphine)ligand for both metals affording optically active 2,3-butadienylα-amino acid derivatives in high to excellent yields with excellent enantioselectivities has been developed. | Junzhe Xiao Haibo Xu Xiaohong Huo Wanbin Zhang Shengming Ma | 2021 | Chinese Journal of Chemistry2021，39，7： | 1 |
| 13 | White microcavity organic light-emitting diode based on one emitting material显示文摘 | Chunyu Zhang Xingyuan Liu Li Qin Wanbin Zhu Lijun Wang | 2006 | Journal of Luminescence2006，，： | 1 |
| 14 | A Pd(Ⅱ)-Catalyzed Oxidative Cyclization for the Preparation of AryI-Fused Six-Membered Nitrogen Heterocycles with 2-Acetoxy Functionality显示文摘Pd (II ) 催化 olefinic tosylamides 的氧化环合为准备被开发熔化芳基并且包含 N 六成员的 heterocycles。在优化条件下面,反应继续了高活动和选择,与多达 83% 的收益被获得。这个过程向一条灵巧、有效的线路提供到上述的 heterocycles 2-acetoxy 功能。 | Xiaolei Wang Zhengxing Wu Xiaowen Zhu Chenghao Ye Feng Jiang Wanbin Zhang | 2013 | Chinese Journal of Chemistry2013，31，1： | 1 |
| 15 | Synthesis of Chiral Hydantoins and Thiazolidinediones via Iridium-Catalyzed Asymmetric Hydrogenation显示文摘Herein,we report an iridium-catalyzed asymmetric hydrogenation of hydantoin and thiazolidinedione derived exocyclic alkenes using our developed BiphPHOX as a ligand.The transformation shows good functional group tolerance,and gives the hydrogenated prod-ucts with excellent yields(up to 99%)and enantioselectivities(up to 98%ee).A gram-scale reaction was also carried out,and pro-vided the hydrogenated product in excellent yield with no erosion in enantioselectivity.Finally,the transformation of the hydrogen-ated product provided an efficient approach for the synthesis of the intermediate of a HIV protease inhibitor. | Yu Nie Jing Li Qianjia Yuan Wanbin Zhang | 2022 | Chinese Journal of Chemistry2022，40，7： | 0 |
| 16 | Convenient synthesis of tropos phosphine-oxazoline ligands显示文摘Tropos phosphine-oxazoline ligands have shown interesting coordination behavior and excellent chiral inducing ability in asymmetry catalysis.Here we present a convenient and economic route for the synthesis of this type of ligands.According to this new route,the ligands with different electronic and steric properties have been prepared successfully. | LIU YuanYuan YANG GuoQiang YAO DongMei TIAN FengTao ZHANG WanBin | 2011 | Science China Chemistry2011，54，1： | 0 |
| 17 | Palladium-Catalyzed Long-Range Isomerization of Aryl Olefins显示文摘Long-range olefin isomerization could lead to the remote functionalization of hydrocarbon chains,which is advantageous with regards to atom-,step-,and redox economy.However,present methodologies for long-range olefin isomerization are mainly focused on heteroatom directed remote olefin migration;studies using aryl groups as the directing group are limited.The limited examples either utilize aryl olefins with special substituted groups on a benzene ring,or use elaborately optimized ligands or co-catalysts to accelerate the isomerization.A more simple catalytic system for general aryl olefins,without the need for special ligands or co-catalysts,was to be developed.Herein,we report a Pd-catalyzed long-range olefin isomerization(up to 15 units)for general aryl olefins via a 1,2-hydrogen shift mechanism.This methodology provides a simple pathway to long-range olefin isomerization without the participation of special ligands or co-catalysts. | Qianyi Ge Jingjie Meng Huikang Liu Zehua Yang Zhengxing Wu Wanbin Zhang | 2022 | Chinese Journal of Chemistry2022，40，19： | 0 |
| 18 | Chiral Bicyclic Imidazole-Catalyzed Direct Enantioselective C-Acetylation of Indolones显示文摘By adjusting the bond angle and stereocontrol substituent of the chiral bicyclic imidazole catalysts,direct enantioselective C-acetylation of indolones and their sequencial pattern have been successfully developed.Indolones bearing a quaternary stereocenter were synthesized with satisfactory yields and excellent enantioselectivities(up to 97%ee).The reaction can be realized with 410 turnover numbers,and the products can be transformed into several functional compounds via simple derivations of the acetyl group. | Muxing Zhou Yashi Zou Lu Zhang Zhenfeng Zhang Wanbin Zhang | 2023 | CCS Chemistry2023，5，2： | 0 |
| 19 | Directional modulation with distributed receiver selection for secure wireless communications显示文摘In this paper, a novel directional modulation with distributed receiver selection(DM-DRS)scheme is proposed for secure wireless communications. In DM-DRS, a particular subset of receivers is activated and part of the information bits are modulated by the index of the activation pattern, in addition to traditional digital modulation. Especially, the scrambling matrix is introduced for the sake of preventing the eavesdropping. Moreover, the performances of bit error rate(BER) in terms of the union bound for both the legitimate user and eavesdropper are respectively derived in the context of an optimal joint maximum likelihood(ML) detector, and the theoretical BER upper bounds are demonstrated to be tight by the numerical results. In the context of the discrete-input and continuous-output system, the ergodic secrecy rates of the legitimate user and the eavesdropper are obtained, the secrecy rate is also quantified. Furthermore,our numerical results exhibit that DM-DRS can achieve an increased transmission rate compared to its traditional directional modulation with cooperative receivers(DM-CR) and spatial and direction modulation(SDM) counterparts, while guaranteeing an improved BER performance. | Hongyan ZHANG Yue XIAO Wanbin TANG Gang WU Hong NIU Xiaotian ZHOU | 2021 | Science China(Information Sciences)2021，64，12： | 0 |
| 20 | Tailoring of a robust asymmetric aramid nanofibers/MXene aerogel film for enhanced infrared thermal camouflage and Joule heating performances显示文摘The development of infrared(IR)surveillance technology has led to a growing interest in thermal camouflage.However,the trade-off relationship between low IR-emissivity and thermal insulation hinders the advance of thermal camouflage materials.Herein,guided by multi-physics simulation,we show a design of asymmetric aramid nanofibers/MXene(ANF/MXene)aerogel film that realizes high-efficient thermal camouflage applications.The rationale is that the asymmetric structure contains a thermal-insulation three-dimensional(3D)network part to prevent effective heat transfer and a low IR-emissivity(~0.3)dense surface layer to suppress radiative heat emission.It is remarkable that the synergy mechanism in the topology structure contributes to over 40%reduction of target radiation temperature.Impressively,the tailored asymmetric ANF/MXene aerogel film also enables sound mechanical properties such as a Young’s modulus of 44.4 MPa and a tensile strength of 1.3 MPa,superior to most aerogel materials.It also exhibits great Joule heating performances including low driving voltage(4 V),fast thermal response(<10 s),and long-term stability,further enabling its versatile thermal camouflage applications.This work offers an innovative design concept to configure multifunctional structures for next-generation thermal management applications. | Wanbin Dang Wei Guo Wenting Chen Qiuyu Zhang | 2024 | Nano Research2024，17，3： | 0 |
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