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| 1 | Microwave-assisted catalytic oxidation of gaseous toluene with a Cu-Mn-Ce/cordierite honeycomb catalyst显示文摘A novel Cu-Mn-Ce/cordierite honeycomb catalyst was prepared by an incipient wetness method and the catalyst was characterized. The active ingredients were present as various spinel species of Cu, Mn and Ce oxides with different valences and they were unevenly dispersed over the surface of the catalyst. The catalytic oxidation of gaseous toluene was primarily investigated using a fixed bed reactor under microwave heating in the continuous flow mode. Under the optimal conditions of 6.7 wt-% loading of the active component, a bed temperature of 200℃, a flow rate of 0.12 m^3 · h^-1 and an initial concentration of toluene of 1000 mg·m^-3, the removal and mineralization efficiencies of toluene were 98% and 70%, respectively. Thus the use of the microwave effectively improved the oxidation of toluene and this is attributed to dipole polarization and hotspot effects. After four consecutive cycles (a total of 1980 min), the Cu-Mn- Ce/cordierite catalyst still exhibited excellent catalytic activity and structural stability, and the toluene removal was higher than 90%. This work demonstrates the possibility of treating volatile organic compounds in exhaust gases by microwave-assisted catalytic oxidation. | Longli Bo Shaoyuan Sun | 2019 | Frontiers of Chemical Science and Engineering2019，13，2： | 11 |
| 2 | CuO/zeolite catalyzed oxidation of gaseous toluene under microwave heating显示文摘为甲苯浪费气体的处理加热的催化氧化和微波的联合进程的开发在这个工作被描述。甲苯,典型有毒的不稳定的有机化合物,通过包含催化剂与硅碳化物混合了的支持沸石的铜氧化物(CuO/zeolite ) 的一个固定的床反应房间被氧化(原文如此) ,优秀吸收微波的材料。目标化合物高效地在温度完成了由的高反应在催化剂的表面上被降级加热微波原文如此。一套试验性的参数例如微波力量,让流动和 CuO 等等的装载尺寸通风,分别地被调查。学习证明这些参数在甲苯降级上有批评影响。在最佳的状况下面, 92% 甲苯被这个联合过程移开,相应于 80%90% TOC 移动率。而且,催化剂甚至在八连续 6-h 跑以后是高度稳定的。最后,甲苯的一条假想降级小径基于从红外线的光谱学分析的煤气的层析团光谱和 Fourier 变换获得的试验性的数据被建议。 | Longli BO Jianbo LIAO Yucai ZHANG Xiaohui WAN Quan YANG | 2013 | Frontiers of Environmental Science & Engineering2013，7，3： | 7 |
| 3 | Microwave assisted wet oxidation of p-nitrophenol显示文摘Aqueous solution of p-nitrophenol (PNP) was treated continuously by microwave assisted wet oxidation while flowing through a granular activated carbon (GAC) fixed bed. PNP was pre-adsorbed onto GAC prior to being put into the reactor so as to prevent PNP adsorption on GAC during microwave irradiation. PNP solutions with different initial concentration (218.6 mg/L and 1200 mg/L) were treated under conditions of microwave power 500 W, liquid flow 6.4 mL/min and air flow 40 mL/min or 60 mL/min. The results indicated that the removal of PNP was higher than 90% and more than 65% PNP was mineralized. Phenol, nitrobenzene, hydroquinone and benzoquinone occurred as course products during the operation process, which were degraded further. The biodegradability of the outflow was improved greatly by microwave assisted wet oxidation. | BO Longli CHEN Shuo QUAN Xie LIU Xitao ZHAO Huimin | 2005 | Science China(Technological Sciences)2005，48，2： | 3 |
| 4 | Biodegradation of trace pharmaceutical substances in wastewater by a membrane bioreactor显示文摘The biodegradation of selected pharmaceutical micropollutants,including two pharmaceuticals with argued biodegradation,was studied by a lab-scale membrane bioreactor.The reaction kinetics and affecting factors were also investigated in this paper.Clofibric acid(CA)with contradictive biodegradation reported was degraded almost completely at different hydraulic retention times(HRTs)after adaptation to microorganisms.The biodegradation of CA was disturbed at low pH operation,while the activity of microorganisms recovered again after pH adjustment to neutral condition.Ibuprofen(IBP)degraded under neutral and acidic conditions.Removals of IBP and CA were zero-order and first-order reactions under high and low initial concentrations,respectively.Carbamazepine and diclofenac were not degraded regardless of HRTs and pH. | Longli BO Taro URASE Xiaochang WANG | 2009 | Frontiers of Environmental Science & Engineering2009，3，2： | 2 |
| 5 | Regeneration of acid orange 7-ex- hausted granular activated carbons with microwave irradiation 显示文摘 | Xie Quan Liu Xitao Bo Longli | 2004 | Water Research2004，38，20： | 1 |
| 6 | Preparation and characteristics of carbon-supported platinum catalyst and its application in the removal of phenolic pollutants in aqueous solution by microwave-assisted catalytic oxidation显示文摘 | Longli Bo Xie Quan Xiaochang Wang | 2008 | Journal of Hazardous Materials2008，，157： | 1 |
| 7 | Regeneration of acid orange 7-exhausted granular activated carbons with microwave irradia- tion显示文摘 | Xie Quan Liu Xiaotao Bo Longli | 2004 | Water Research2004，38，20： | 1 |
| 8 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation显示文摘 | Liu Xitao Quan Xie Bo Longli | 2004 | Carbon2004，，42： | 1 |
| 9 | Simultaneous Pentachlorophenol Decomposition and Granular Activated Ccarbon Regeneration Assisted by Microwave Irradiation显示文摘 | LIU Xi-tao Quan Xie Bo Longli | 2004 | Carbon2004，42，2： | 1 |
| 10 | Temperature measurement of GAC and decomposition of PCP loaded on GAC and GAC-supported copper catalyst in microwave irradiation 显示文摘 | LIU Xitao QUAN Xie BO Longli | 2004 | Applied Catalysis : General2004，264，1： | 1 |
| 11 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation显示文摘 | Liu Xitao Xie Quan Bo Longli | 2004 | Carbon2004，42，2： | 1 |
| 12 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation显示文摘 | Liu Xitao Quan Xie Bo Longli et at | 2004 | Carbon2004，42，2： | 1 |
| 13 | Degradation of p-nitrophenol in aqueous solution by microwave assisted oxidation process through a granular activated carbon fixed bed显示文摘 | Xie Quan Shuo Chen | 2006 | WATERRESEARCH2006，40，： | 1 |
| 14 | Simultaneous pentachlorophenol decomposition and granuual activated carbon regeneration assisted by microwave irradiation 显示文摘 | Xitao Liu Xie Quan Longli Bo Shuo Chen Yazhi Zhao | 2004 | Cabon2004，42，： | 1 |
| 15 | Regeneration of acid orange 7-exhausted granular activated carbons with microwave irradiation显示文摘 | Xie Quan Xitao Liu Longli Bo Shuo Chen Yazhi Zhao Xinyi Cui | 2004 | Water Research2004，，20： | 1 |
| 16 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation 显示文摘 | Liu Xitao Quan Xie Bo Longli | 2004 | Carbon2004，，42： | 1 |
| 17 | Regeneration of acid orange 7 -exhausted grarmlar activated carbons withmicrowave irradiation显示文摘 | Xie Quan Xitao Liu Longli Bo | 2004 | Water Research2004，38，： | 1 |
| 18 | Simultaneous penta- chlorophenol decomposition and granular activated carbon re- generation assisted by microwave irradiation 显示文摘 | LIU Xitao XIE Quan BO Longli | 2004 | Carbon2004，42，2： | 1 |
| 19 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation 显示文摘 | Liu Xitao Quan Xie Bo LongLi | 2004 | Carbon2004，42，2： | 1 |
| 20 | Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by microwave irradiation 显示文摘 | LIU Xitao QUAN Xie BO Longli | 2004 | Carbon2004，42，2： | 1 |
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