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| 1 | Homogeneous bottom-growth of lithium metal anode enabled by double-gradient lithiophilic skeleton显示文摘Lithium(Li) metal is considered as the most promising anode material for the next-generation high performance Li batteries.However,the uncontrollable dendritic growth impedes its commercial application.Herein,we design a 3 D Si@carbon nanofibers(CNFs)@ZnO-ZnO-Cu skeleton(SCZ) for guiding the homogeneous bottom-growth of Li metal.The top LixSi@CNFs and bottom LiyZn@CNFs layers could form conductivity and overpotential gradient to avoid the 'top-growth' of Li metal.Moreover,the top lithiophilic LixSi@CNFs layer could regulate the nucleation and deposition of Li-ions even if the lithium dendrites grow out of the skeleton under high capacity Li deposition(30 mAh cm^(-2)).As a result,the SCZ-Li||LiFePO_(4) full cell delivers a high capacity of ~104 mAh g^(-1)(~94.82% capacity retention) after 2000 cycles at 5 C, elucidating the potential application of the 3 D double-gradient Li metal composite anode. | Li Zhang Hongfei Zheng Ben Liu Qingshui Xie Qiulin Chen Liang Lin Jie Lin Baihua Qu Laisen Wang Dong-Liang Peng | 2021 | Journal of Energy Chemistry2021，30，6： | 5 |
| 2 | Flexible organic thin-film transistors based on poly(3-hexylthiophene) films for nitrogen dioxide detection显示文摘Flexible nitrogen dioxide(NO_2) gas sensors based on organic thin-film transistors(OTFTs) were developed in this work, in which conductive indium tin oxide(ITO) coated polyethylene naphthalene-2,6-dicarboxylate(PEN) was designed for the flexible substrates, and poly methyl methacrylate(PMMA) and poly(3-hexylthiophene)(P3HT) was spin-coated as the gate dielectric layer and spray-deposited as the active layer, respectively. The effects of PMMA concentrations and P3HT solution volume on performances of flexible OTFTs were systematically investigated. The results showed that the optimized flexible OTFT exhibited high field-effect mobility(9.51×10^(–3) cm^2/(V s) at a gate bias of –50 V) and excellent response characteristics,including high sensitivity(up to 0.169 ppm^(–1)), good repeatability and selectivity. The flexibility of the developed OTFT sensor was also investigated, and the results showed that the electrical and gas-sensing properties were affected by the bending cycles,thus further work should be done for improving the flexibility of the sensor. This work provides an effective approach in developing high performance flexible OTFT NO_2 gas sensor. | YANG Jing XIE GuangZhong SU YuanJie ZHANG QiuPing DU HongFei TAI HuiLing DU XiaoSong JIANG YaDong | 2018 | Science China(Technological Sciences)2018，61，11： | 3 |
| 3 | The first pulsar discovered by FAST显示文摘To assist with the commissioning [1] of the Five-hundredmeter Aperture Spherical radio Telescope (FAST), we performed a pulsar search, with the primary goal of developing and testing the pulsar data acquisition and processing pipelines. We tested and used three pipelines, two (Pl and P2 hereafter) searched for the periodic signature of pulsars whereas the other one was used to search for bright single pulses (P3 hereafter). | Lei Qian ZhiChen Pan Di Li George Hobbs WeiWei Zhu Pei Wang ZhiJie Liu YouLing Yue Yan Zhu HongFei Liu DongJun Yu JingHai Sun Peng Jiang GaoFeng Pan Hui Li HengQian Gan Rui Yao XiaoYao Xie Fernando Camilo Andrew Cameron Lei Zhang Shen Wang FAST Collaboration | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，5： | 3 |
| 4 | 3D uniform nitrogen-doped carbon skeleton for ultra-stable sodium metal anode显示文摘Sodium metal batteries are arousing extensive interest owing to their high energy density,low cost and wide resource.However,the practical development of sodium metal batteries is inherently plagued by the severe volume expansion and the dendrite growth of sodium metal anode during long cycles under high current density.Herein,a simple electrospinning method is applied to construct the uniformly nitrogen-doped porous carbon fiber skeleton and used as three-dimensional(3D)current collector for sodium metal anode,which has high specific surface area(1,098 m^2/g)and strong binding to sodium metal.As a result,nitrogen-doped carbon fiber current collector shows a low sodium deposition overpotential and a highly stable cyclability for 3,500 h with a high coulombic effciency of 99.9%at 2 mA/cm^2 and 2 mAh/cm^2.Moreover,the full cells using carbon coated sodium vanadium phosphate as cathode and sodium pre-plated nitrogen-doped carbon fiber skeleton as hybrid anode can stably cycle for 300 times.These results illustrate an effective strategy to construct a 3D uniformly nitrogen-doped carbon skeleton based sodium metal hybrid anode without the formation of dendrites,which provide a prospect for further development and research of high performance sodium metal batteries. | Ben Liu Danni Lei Jin Wang Qingfei Zhang Yinggan Zhang Wei He Hongfei Zheng Baisheng Sa Qingshui Xie Dong-Liang Peng Baihua Qu | 2020 | Nano Research2020，13，8： | 3 |
| 5 | A randomized, multi-central, controlled study of patients with hepatitis B e antigen-positive chronic hepatitis B treated by adefovir dipivoxil or adefovir dipivoxil plus bicyclol显示文摘 | Wen Xie Guangfeng Shi Hongfei Zhang Guiming Zhao Zujiang Yu Zhenwei Lang Hong Zhao Jie Yan Jun Cheng | 2012 | Hepatology International2012，，2： | 1 |
| 6 | Adsorption behaviors of gas molecules on the surface of ZnO nanocrystals under UV irradiation显示文摘A UV-activated room temperature chemiresistive gas sensor based on ZnO nanocrystals film was fabricated. Its gas sensing properties under various conditions were also investigated in detail. The results shed new insight into the adsorption behaviors of gas molecules on the surface of ZnO nanocrystals under UV irradiation. The chemisorbed oxygen species(O^-2(ads)(hv)) induced by UV light govern the adsorption and desorption ways of other gas molecules on the surface of ZnO nanocrystals, which is dependent on the electron affinity of gas molecules. Gas molecules with higher electron affinity than oxygen molecules can be adsorbed on the surface by the competitive adsorption way, extracting electrons from the surface. Gas molecules with lower electron affinity than oxygen molecules are attracted by the adsorbed O^-2(ads)(hv)layer, releasing electrons to the surface. These processes can influence the gas sensing properties of the sensor. Our findings will pave the way for the fundamental understanding and design of UV-activated gas sensor in the future. | ZHANG QiuPing XIE GuangZhong DU HongFei YANG Jing SU YuanJie TAI HuiLing XU Ming ZHAO Kang | 2019 | Science China(Technological Sciences)2019，62，12： | 1 |
| 7 | Facile biphasic catalytic process for conversion of monoterpenoids to tricyclic hydrocarbon biofuels显示文摘Terpenoids have drawn much attention to scientists in synthesizing high-performance bio-jet fuels due to their ring structures,which feature potential high densities.Here,a facile biphasic catalytic process has been developed for the production of high-density tricyclic hydrocarbon biofuels from a monoterpenoid,1,8-cineole,using sulfuric acid(H2SO4)as the homogeneous catalyst.A^100%conversion of 1,8-cineole and a>40%carbon yield of cyclic dimers were achieved at 100℃within two hours.The mechanism for the acid-catalyzed conversion of 1,8-cineole to cyclic hydrocarbon dimers were explored.In particular,the formation of the diene intermediates and the following dimerization of dienes was essential to synthesize tricyclic terpene dimers.The biphasic catalytic process accelerated the deoxygenation rate and enabled the dimerization with the aid of organic solvent while controlling the reaction rates to avoid the formation of solid residues.Moreover,this process also facilitated the product separation by organic solvent extraction while enabling easy recycle of the homogenous catalysts. | Shaoqu Xie Trong HHuynh Peiyong Qin Tianwei Tan Hongfei Lin | 2020 | Journal of Energy Chemistry2020，29，10： | 1 |
| 8 | Evaluation of antioxidant activities of principal carotenoids available in water spinach (lpomoea aquatica)显示文摘 | FU Hongfei XIE Bijun MA Shaojun | 2011 | Journal of Food Composition and Analysis2011，24，2： | 1 |
| 9 | Effect of esterification with fatty acid of β-cryptoxanthin on its thermal stability and antioxidant activity by chemiluminescence method显示文摘 | HongFei Fu BiJun Xie Gang Fan ShaoJun Ma XinRong Zhu SiYi Pan | 2010 | Food Chemistry2010，，3： | 1 |
| 10 | Polyvinylpyrrolidone/graphene oxide thin films coated on quartz crystal microbalance electrode for NH_3 detection at room temperature显示文摘In this paper, composite film based on polyvinylpyrrolidone(PVP)/graphene oxide(GO) was fabricated by spray method on AT-cut 9.986 MHz quartz crystal microbalance(QCM) for NH_3 sensing. The thin films were characterized by scanning electron microscope(SEM), Fourier transform infrared spectroscopy(FTIR) and ultraviolet-visible spectroscopy(UV-VIS) to investigate the morphologies and the composition contents, respectively. The experimental results reveal that PVP/GO based sensor holds higher sensitivity, larger responsiveness and smaller baseline drift than those based on pure PVP at room temperature. Besides, the prepared sensor exhibits greater response to NH_3 than other gases such as CO, CO_2 and NO_2 at the same concentration. The good linearity, reproducibility and stability demonstrate the practicability of PVP/GO hybrid film in detecting NH_3. | MA XingFang XIE GuangZhong SU YuanJie DU HongFei XIE Tao JIANG YaDong | 2016 | Science China(Technological Sciences)2016，59，9： | 1 |
| 11 | Evaluation of an- tioxidant activities of principal carotenoids available in water spinach ( Ipomoea aquatica) 显示文摘 | Hongfei Fu Bijun Xie Shaojun Ma | 2011 | Journal of Food Composition and Analysis2011，24，： | 1 |
| 12 | Polyethylene glycol/polylactic acid block co‐polymers as solid–solid phase change materials显示文摘Phase change materials(PCMs)are promising thermal energy storage materials due to their high specific latent heat.Conventional PCMs typically exploit the solid–liquid(s–l)transition.However,leakage and leaching are common issues for solid–liquid PCMs,which have to be addressed before usage in practical applications.In contrast,solid–solid(s–s)PCMs would naturally overcome these issues due to their inherent form stability and homogeneity.In this study,we report a new type of s–s PCM based on chemically linked polyethylene glycol(PEG,the PCM portion)with polylactic acid(PLA,the support portion)in the form of a block co‐polymer.Solid‐solid latent heat of up to 56 J/g could be achieved,with melting points of between 44°C and 55°C.For comparison,PEG was physically mixed into a PLA matrix to form a PEG:PLA composite.However,the composite material saw leakage of up to 9%upon heating,with a corresponding loss in thermal storage capacity.In contrast,the mPEG/PLA block co‐polymers were found to be completely homogeneous and thermally stable even when heated above its phase transition temperature,with no observable leakage,demonstrating the superiority of chemical linking strategies in ensuring form stability. | Xiang YDSoo Joseph K.Muiruri Jayven CCYeo Zhuang MPng Anqi Sng Huiqing Xie Rong Ji Suxi Wang Hongfei Liu Jianwei Xu Xian JLoh Qingyu Yan Zibiao Li Qiang Zhu | 2023 | SmartMat2023，4，3： | 1 |
| 13 | Topological photonic crystals:a review显示文摘The field of topological photonic crystals has attracted growing interest since the inception of optical analog of quantum Hall effect proposed in 2008.Photonic band structures embraced topological phases of matter,have spawned a novel platform for studying topological phase transitions and designing topological optical devices.Here,we present a brief review of topological photonic crystals based on different material platforms,including all-dielectric systems,metallic materials,optical resonators,coupled waveguide systems,and other platforms.Furthermore,this review summarizes recent progress on topological photonic crystals,such as higherorder topological photonic crystals,non-Hermitian photonic crystals,and nonlinear photonic crystals.These studies indicate that topological photonic crystals as versatile platforms have enormous potential applications in maneuvering the flow of light. | Hongfei WANG Samit Kumar GUPTA Biye XIE Minghui LU | 2020 | Frontiers of Optoelectronics2020，13，1： | 1 |
| 14 | Interfacial ion regulation on 2D layered double hydroxide nanosheets for enhanced thermal insulation显示文摘Exploring new strategies to broaden the upper/lower limit of thermal conductivity is of great interest to develop thermal management materials that can adapt to extreme environments.In this work,we employ an interfacial ion regulation to enhance the thermal insulation performance of 2D layered double hydroxide nanosheets.The introduction of interfacial ion enlarges the interplanar spacing of Co(OH)_(2) nanosheets from 4.64 to 8.05 ?,which reduces phonon scattering length perpendicular to the two-dimensional plane and leads to enhanced interlayer thermal insulation.The interfacial ion-regulated Co(OH)_(2)(named as Co(OH)_(2)-M^(x-)) exhibits 3-fold enhancement of thermal insulation through decreasing the thermal conductivity to as low as 0.15 W m^(-1) K^(-1),which is among the top values in 2D solid materials.We anticipate that interfacial ion regulation for 2D nanosheets paves a new avenue to break through the thermal insulation limit. | Chun Wang Hengyu Xu Han Cheng Hao Yu Si Liu Wenjie Wang Ruilin Yuan Hongfei Liu Tianpei Zhou Wangsheng Chu HengAn Wu Yi Xie Changzheng Wu | 2022 | Science China Chemistry2022，65，5： | 0 |
| 15 | Field distribution of the Z_(2)topological edge state revealed by cathodoluminescence nanoscopy显示文摘Photonic topological insulators with robust boundary states can enable great applications for optical communication and quantum emission,such as unidirectional waveguide and single-mode laser.However,because of the diffraction limit of light,the physical insight of topological resonance remains unexplored in detail,like the dark line that exists with the crys-talline symmetry-protected topological edge state.Here,we experimentally observe the dark line of the Z_(2)photonic topo-logical insulator in the visible range by photoluminescence and specify its location by cathodoluminescence characteriza-tion,and elucidate its mechanism with the p-d orbital electromagnetic field distribution which calculated by numerical sim-ulation.Our investigation provides a deeper understanding of Z_(2)topological edge states and may have great signific-ance to the design of future on-chip topological devices. | Xiao He Donglin Liu Hongfei Wang Liheng Zheng Bo Xu Biye Xie Meiling Jiang Zhixin Liu Jin Zhang Minghui Lu Zheyu Fang | 2022 | Opto-Electronic Advances2022，5，4： | 0 |
| 16 | TiO_(2) nanofiber-supported copper nanoparticle catalysts for highly efficient methane conversion to C1 oxygenates under mild conditions显示文摘The selective oxidation of methane under mild conditions remains the“Holy Grail of Catalysis”.The key to activating methane and inhibiting over-oxidation of target oxygenates lies in designing active centers.Copper nanoparticles were loaded onto TiO_(2) nanofibers using the photo-deposition method.The resulting catalysts were found to effectively convert methane into C1 oxygenated products under mild conditions.Compared with previously reported catalysts,it delivers a superior performance of up to 2510.7 mmol·g_(Cu)^(-1)·h^(-1) productivity with a selectivity of around 100%at 80℃for 5 min.Microstructure characterizations and density functional theory(DFT)calculations indicate that TiO_(2) in the mixed phase of anatase and rutile significantly increases the Cu^(+)/CuO ratio of the supported Cu species,and this ratio is linearly related to the formation rate of oxygen-containing species.The CuI site promotes the generation of active O species from H_(2)O_(2) dissociation on Cu_(2)O(111).These active O species reduce the energy barrier for breaking the C-H bond of CH_(4),thus boosting the catalytic activity.The methane conversion mechanism was proposed as a methyl radical pathway to form CH_(3)OH and CH_(3)OOH,and then the generated CH_(3)OH is further oxidized to HOCH_(2)OOH. | Wencui Li Yu Ren Zean Xie Yipeng Wang Hang Zhang Dianxiang Peng Hengfang Shen Hongfei Shi Jiaxin Cai Peng Wang Tongxin Zhang Zhen Zhao | 2024 | Nano Research2024，17，5： | 0 |
| 17 | Transpiration-inspired Capillary for Synchronous Synthesis and Patterning of Silver Nanoparticles显示文摘Traditional synthesis strategy of nanomaterials with complicated process and high cost limits their applications.Here,we propose a facile process for the synchronous synthesis and patterning of silver nanoparticles(Ag NPs)through the self-driven microchannel reactor with the capillary effect inspired by transpiration.The evaporation contributes to capillary and accumulation effects in the microchannels.The silver reactant-containing droplets can be spontaneously divided and distributed in multiple microchannels during the whole fabrication process by the capillary effect.The newly formed Ag NPs at the gas-liquid interface can be assembled on both sides of the microchannels by the accumulation effect.The capillary effect decreases the disturbances,which ensures the uniformity of the patterning.By the combination of microchannels with different widths,various Ag NPs-assembled patterns with stable electrical properties are achieved.This efficient strategy with a simple fabrication procedure is towards the technological engineering of nanoscale architected materials. | CHEN Bingda ZHANG Zelong SU Meng QIN Feifej PAN Qi XIE Daixi YANG Xu ZHANG Kun ZHANG Zeying XIE Hongfei CARMELIET Jan SONG Yanlin | 2023 | Chemical Research in Chinese Universities2023，39，1： | 0 |
| 18 | Smartphone-based rapid and visual pathological diagnosis of glioma using perovskite probes显示文摘Histopathology plays a great role in diagnosing various diseases,which is considered as a golden standard for tumor identification.The tissue constituents must be stained by visible labels for microscopic analysis by medical experts.However,this process is time-consuming,labor-intensive,and expensive,which requires rapid pathological approaches for diagnosis in the operating room.Here,we present an easy-to-process and high-performance perovskite biological probes for rapid and visual pathological diagnosis of glioma.Perovskite quantum dots can be encapsulated by the copolymer into nanocrystals(PNCs)with a diameter of 100 nm,which is modified with chlorotoxin to achieve the specific recognition of glioma.Benefiting from the super photoluminescence quantum yield(above 93%)of EVA@PNCs aqueous solution,the glioma can be clearly imaged and captured via a smartphone under the excitation of a handheld UV lamp.To demonstrate the visualization and efficiency of PNC probes,different malignant grades of brain tumor sections can be distinguished in no more than 5 min.This strategy provides a general auxiliary diagnosis platform for achieving the histopathology analysis near the operating bed,which is currently not feasible with standard histochemical staining methods. | Dongdong Wu Jimei Chi Junzhen Fan Lijun Cheng Xuning Wang Xu Yang Meng Zhang Zewei Lian Zengqi Huang Huadong Wang Hongfei Xie Sisi Chen Qi Pan Zeying Zhang Bingda Chen Guochen Sun Bainan Xu Meng Su Yanlin Song | 2023 | InfoMat2023，5，11： | 0 |
| 19 | Laboratory Study on CR/SBS Modified Asphalt:Preparation and Performance Characterization显示文摘Crumble rubber(CR)can be used to prepare CR and styrene-butadiene-styrene(SBS)composite modified asphalt with a good high-and low-temperature performance,meanwhile the addition of CR could work as the substitute for SBS and help reduce the content of SBS.This study contains three main parts:effect of preparation and effect of material composition as well as rheological performance characterization.Factors during the preparation,including shearing temperature,shearing time,mixing time and swelling time,were selected,while base binder,CR content,CR particle size and SBS content in material composition were considered.The effects of these factors were assessed in terms of the conventional performance(penetration,softening point,ductility and storage stability).After identifying these effects,the sample of CR and SBS modified asphalt at the selected preparing condition and material composition(CR/SBSMA)was made,and the corresponding SBS modified and CR modified asphalt(SBSMA and CRMA)were produced for the comparing reason.Subsequently,temperature sweeps from 0℃ to 80℃ were utilized to depict the viscoelasticity of these modified asphalt binders by complex modulus and phase angle.Multiple stress creep recovery tests(MSCR)at 64℃ and bending beam rheometer tests(BBR)at various low temperatures were employed to evaluate the high-and low-temperature performance,respectively.Results highlight that that CR/SBSMA could exhibit an excellent high-temperature performance(better than SBSMA),and a good low-temperature performance(reaching the level of base binder). | Liang Song Guoqiang Zhang Hongfei Xie Jie Gao | 2022 | Journal of Renewable Materials2022，10，6： | 0 |
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